Rational Design of a High Performance and Robust Solar Evaporator via 3D-Printing Technology

被引:109
作者
Chaule, Sourav [1 ]
Hwang, Jongha [1 ]
Ha, Seong-Ji [1 ]
Kang, Jihun [1 ]
Yoon, Jong-Chul [1 ]
Jang, Ji-Hyun [1 ]
机构
[1] Ulsan Natl Inst Technol UNIST, Sch Energy & Chem Engn, 50 UNIST Gil, Ulsan 44919, South Korea
关键词
anti-fouling effect; double layered photoabsorber; light harvesting; solar desalination; SEAWATER DESALINATION; WATER-PURIFICATION; EFFICIENT; DRIVEN; NANOPARTICLES; MEMBRANE;
D O I
10.1002/adma.202102649
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Utilizing the broad-band solar spectrum for sea water desalination is a promising method that can provide fresh water without sophisticated infrastructures. However, the solar-to-vapour efficiency has been limited due to the lack of a proper design for the evaporator to deal with either a large amount of heat loss or salt accumulation. Here, these issues are addressed via two cost-effective approaches: I) a rational design of a concave shaped supporter by 3D-printing that can promote the light harvesting capacity via multiple reflections on the surface; II) the use of a double layered photoabsorber composed of a hydrophilic bottom layer of a polydopamine (PDA) coated glass fiber (GF/C) and a hydrophobic upper layer of a carbonized poly(vinyl alcohol)/polyvinylpyrrolidone (PVA/PVP) hydrogel on the supporter, which provides competitive benefit for preventing deposition of salt while quickly pumping the water. The 3D-printed solar evaporator can efficiently utilize solar energy (99%) with an evaporation rate of 1.60 kg m(-2) h(-1) and efficiency of 89% under 1 sun irradiation. The underlying reason for the high efficiency obtained is supported by the heat transfer mechanism. The 3D-printed solar evaporator could provide cheap drinking water in remote areas, while maintaining stable performance for a long term.
引用
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页数:10
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