Modeling the influence of biogenic volatile organic compound emissions on ozone concentration during summer season in the Kinki region of Japan

被引:26
作者
Bao, Hai [2 ]
Shrestha, Kundan Lal [1 ]
Kondo, Akira [1 ]
Kaga, Akikazu [1 ]
Inoue, Yoshio [1 ]
机构
[1] Osaka Univ, Grad Sch Engn, Div Sustainable Energy & Environm Engn, Suita, Osaka 5650871, Japan
[2] Inner Mongolia Normal Univ, Chem & Environm Sci Coll, Hohhot 010022, Peoples R China
关键词
Biogenic volatile organic compound; Ozone; MM5; CMAQ; Growth chamber; RATE VARIABILITY; ISOPRENE; POLLUTION;
D O I
10.1016/j.atmosenv.2009.10.021
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Tropospheric ozone adversely affects human health and vegetation, and biogenic volatile organic compound (BVOC) emission has potential to influence ozone concentration in summer season. In this research, the standard emissions of isoprene and monoterpene from the vegetation of the Kinki region of Japan, estimated from growth chamber experiments, were converted into hourly emissions for July 2002 using the temperature and light intensity data obtained from results of MM5 meteorological model. To investigate the effect of BVOC emissions on ozone production, two ozone simulations for one-month period of July 2002 were carried out. In one simulation, hourly BVOC emissions were included (1310), while in the other one, BVOC emissions were not considered (NOBIO). The quantitative analyses of the ozone results clearly indicate that the use of spatio-temporally varying BVOC emission improves the prediction of ozone concentration. The hourly differences of monthly-averaged ozone concentrations between BIO and NOBIO had the maximum value of 6 ppb at 1400 JST. The explicit difference appeared in urban area, though the place where the maximum difference occurred changed with time. Overall, BVOC emissions from the forest vegetation strongly affected the ozone generation in the urban area. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码:421 / 431
页数:11
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