Removal of Methylene Blue by lava adsorption and catalysis oxidation

被引:10
作者
Ma, Jianfeng [1 ]
Zhang, Jinbao [1 ]
Li, Dinglong [1 ]
机构
[1] Jiangsu Polytech Univ, Coll Environm & Safety Engn, Changzhou 213164, Jiangsu, Peoples R China
关键词
adsorption; catalysis oxidation; Methylene Blue; lava; wastewater treatment; LOW-COST ADSORBENTS; AQUEOUS-SOLUTIONS; MODIFIED ZEOLITES; REACTIVE DYE; BASIC-DYES; CONGO RED; WASTE; SHELL; EQUILIBRIUM; DEGRADATION;
D O I
10.1080/09593330903453244
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Adsorption has been found to be effective for the removal of dyes from effluent; however, the contaminant will cause secondary pollution if it is not properly treated. In this paper, the ability of lava as a low-cost adsorbent and catalyst for the removal of a commercial dye, Methylene Blue (MB), from aqueous solution has been investigated under various experimental conditions. It was found that lava had a high efficiency (more than 98%) for MB removal by adsorption. The adsorption equilibrium data can be fitted well by the Langmuir adsorption isotherm model. The adsorption kinetics was shown to be pseudo-second-order. After adsorption the contaminant could be catalysis oxidized by lava with the aids of H(2)O(2) and ultrasound. The result showed that 95% of the MB could be decomposed in 100 min with the aid of ultrasound at 85 W/cm(2). Overall, this study demonstrates lava as a promising material for wastewater treatment to remove and decompose dyes in a single treatment step.
引用
收藏
页码:267 / 276
页数:10
相关论文
共 34 条
[1]   Adsorption of Congo red from aqueous solution onto calcium-rich fly ash [J].
Acemioglu, B .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2004, 274 (02) :371-379
[2]   Batch kinetic study of sorption of methylene blue by perlite [J].
Acemioglu, B .
CHEMICAL ENGINEERING JOURNAL, 2005, 106 (01) :73-81
[3]   Investigation on the adsorption capability of egg shell membrane towards model textile dyes [J].
Arami, Mokhtar ;
Limaee, Nargess Yousefi ;
Mahmoodi, Niyaz Mohammad .
CHEMOSPHERE, 2006, 65 (11) :1999-2008
[4]   The removal of reactive azo dyes by natural and modified zeolites [J].
Armagan, B ;
Özdemir, O ;
Turan, M ;
Çelik, MS .
JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY, 2003, 78 (07) :725-732
[5]   Acid dyes removal using low cost adsorbents [J].
Aydin, AH ;
Bulut, Y ;
Yavuz, Ö .
INTERNATIONAL JOURNAL OF ENVIRONMENT AND POLLUTION, 2004, 21 (01) :97-104
[6]   Removal of congo red dye from water using carbon slurry waste [J].
Bhatnagar, A. ;
Jain, A. K. ;
Mukul, M. K. .
ENVIRONMENTAL CHEMISTRY LETTERS, 2005, 2 (04) :199-202
[7]   Adsorption of gases in multimolecular layers [J].
Brunauer, S ;
Emmett, PH ;
Teller, E .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1938, 60 :309-319
[8]   Removal of Methylene Blue from aqueous solution by adsorption on sand [J].
Bukallah, Saeed B. ;
Rauf, M. A. ;
AlAli, S. S. .
DYES AND PIGMENTS, 2007, 74 (01) :85-87
[9]   Adsorption of basic dye onto activated carbon prepared from durian shell: Studies of adsorption equilibrium and kinetics [J].
Chandra, Thio Christine ;
Mirna, M. M. ;
Sudaryanto, Y. ;
Ismadji, S. .
CHEMICAL ENGINEERING JOURNAL, 2007, 127 (1-3) :121-129
[10]   Surface charge evolution of mineral-organic complexes during pedogenesis in Hawaiian basalt [J].
Chorover, J ;
Amistadi, MK ;
Chadwick, OA .
GEOCHIMICA ET COSMOCHIMICA ACTA, 2004, 68 (23) :4859-4876