Tracing sources of nitrate using water chemistry, land use and nitrogen isotopes in the Ganjiang River, China

被引:13
作者
Wang, Peng [1 ,2 ]
Liu, Junzheng [1 ,2 ]
Qi, Shuhua [1 ,2 ]
Wang, Shiqin [3 ]
Chen, Xiaoling [4 ]
机构
[1] Jiangxi Normal Univ, Minist Educ, Key Lab Poyang Lake Wetland & Watershed Res, Nanchang, Jiangxi, Peoples R China
[2] Jiangxi Normal Univ, Sch Geog & Environm, Nanchang, Jiangxi, Peoples R China
[3] Chinese Acad Sci, Inst Genet & Dev Biol, Key Lab Agr Water Resources, Shijiazhuang, Hebei, Peoples R China
[4] Wuhan Univ, State Key Lab Informat Engn Surveying Mapping & R, Wuhan, Hubei, Peoples R China
基金
中国国家自然科学基金;
关键词
Domestic and industrial sewage; fertilizer; Ganjiang River; isotope geochemistry; land use; nitrate source; nitrogen-15; water chemistry; STABLE-ISOTOPES; MISSISSIPPI RIVER; POYANG LAKE; SEINE RIVER; FRESH-WATER; DENITRIFICATION; STREAMS; TRANSFORMATIONS; QUALITY; OXYGEN;
D O I
10.1080/10256016.2017.1328417
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
In this work, we traced sources of nitrate in the Ganjiang River, a major tributary of Yangtze River, China, by analysing the water chemistry, nitrogen isotopes and land use. Water samples from 20 sites in the main stream and tributaries were collected in the dry and wet seasons. The delta N-15-NO3- ranged from 0.97 to 8.60%, and was significantly higher in the wet season than in the dry season, and significantly higher in tributaries than in the main stream. In the dry season, NO3- concentrations and delta N-15-NO3- were significantly negatively correlated with forest and grassland areas, and positively correlated with paddy field and residential area. However, most of the correlations were not significant in the wet season. The results showed that fertilizer was the main source of nitrate in the Ganjiang River, and domestic sewage was important in the dry season, but its contribution was lower than that in other rivers in the Yangtze Basin. In the wet season, the intensified nitrogen cycle caused by high temperature and the mixing effect caused by rainfall made it difficult to trace nitrate sources using delta N-15-NO3- and land use.
引用
收藏
页码:539 / 551
页数:13
相关论文
共 45 条
[1]   Effect of stream channel size on the delivery of nitrogen to the Gulf of Mexico [J].
Alexander, RB ;
Smith, RA ;
Schwarz, GE .
NATURE, 2000, 403 (6771) :758-761
[2]   Chemical and isotopic evidence of nitrogen transformation in the Mississippi River, 1997-98 [J].
Battaglin, WA ;
Kendall, C ;
Chang, CCY ;
Silva, SR ;
Campbell, DH .
HYDROLOGICAL PROCESSES, 2001, 15 (07) :1285-1300
[3]   Nitrogen removal in streams of agricultural catchments - A literature review [J].
Birgand, Francois ;
Skaggs, R. Wayne ;
Chescheir, George M. ;
Gilliam, J. Wendell .
CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY, 2007, 37 (05) :381-487
[4]   Nitrate stable isotopes: tools for determining nitrate sources among different land uses in the Mississippi River Basin [J].
Chang, CCY ;
Kendall, C ;
Silva, SR ;
Battaglin, WA ;
Campbell, DH .
CANADIAN JOURNAL OF FISHERIES AND AQUATIC SCIENCES, 2002, 59 (12) :1874-1885
[5]   Nitrate sources and watershed denitrification inferred from nitrate dual isotopes in the Beijiang River, south China [J].
Chen, Fajin ;
Jia, Guodong ;
Chen, Jianyao .
BIOGEOCHEMISTRY, 2009, 94 (02) :163-174
[6]   Assessment of the sources and transformations of nitrogen in a plain river network region using a stable isotope approach [J].
Ding, Jingtao ;
Xi, Beidou ;
Xu, Qigong ;
Su, Jing ;
Huo, Shouliang ;
Liu, Hongliang ;
Yu, Yijun ;
Zhang, Yanbo .
JOURNAL OF ENVIRONMENTAL SCIENCES, 2015, 30 :198-206
[7]   Hydrological Effects on Relationships Between 15N of River Nitrate and Land Use in a Rural River Basin, Western Japan [J].
Ide, J. ;
Somura, H. ;
Nakamura, T. ;
Mori, Y. ;
Takeda, I. ;
Nishida, K. .
RIVER RESEARCH AND APPLICATIONS, 2015, 31 (05) :639-649
[8]   Isotopic composition of nitrate in five German rivers discharging into the North Sea [J].
Johannsen, Astrid ;
Daehnke, Kirstin ;
Emeis, Kay .
ORGANIC GEOCHEMISTRY, 2008, 39 (12) :1678-1689
[9]   Nitrate cycling in streams:: using natural abundances of NO-3-δ15N to measure in-situ denitrification [J].
Kellman, L ;
Hillaire-Marcel, C .
BIOGEOCHEMISTRY, 1998, 43 (03) :273-292
[10]  
Kendall C, 1998, ISOTOPE TRACERS IN CATCHMENT HYDROLOGY, P519