Computational Fluid Dynamics Analysis of the Micromixing Efficiency in a Rotating-Packed-Bed Reactor

被引:53
作者
Guo, Tian-Yu [1 ]
Shi, Xin [1 ]
Chu, Guang-Wen [2 ]
Xiang, Yang [2 ]
Wen, Li-Xiong [1 ,2 ]
Chen, Jian-Feng [1 ,2 ]
机构
[1] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
[2] Beijing Univ Chem Technol, Res Ctr, Minist Educ High Grav Engn & Technol, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
COMPETING REACTION SYSTEM; PROCESS INTENSIFICATION; CFD ANALYSIS; GAS-FLOW; MALDISTRIBUTION; PRECIPITATION; SIMULATION; CONTACTOR; IODIDE; VOLUME;
D O I
10.1021/acs.iecr.6b00213
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Micromixing in rotating-packed-bed (RPB) reactors is of great significance for their process-intensifying performance. On the basis of the iodide-iodate reaction system, a two-dimensional computational framework of RPB was developed to investigate the micromixing efficiency in a RPB. The volume-of-fluid multiphase model, laminar finite-rate model, and the Reynolds stress model were adopted to simulate the volumetric fraction of the liquid phase, the concentration distributions, and the effects of rotating speed and liquid flow velocity on the micromixing performance of a RPB. The computational fluid dynamics results showed that the micromixing and reaction processes occurred mainly in the inlet region of RPB packing, which further confirmed the end effect of the packing. An increase of the rotating speed and liquid flow velocity could remarkably enhance the micromixing efficiency in a RPB. On the basis of the incorporation model, the micromixing time in a RPB was estimated as 0.05-0.30 ms, indicating a remarkably quick micromixing performance.
引用
收藏
页码:4856 / 4866
页数:11
相关论文
共 40 条
[1]  
[Anonymous], 2006, THEOR GUID FLUENT 6
[2]  
[Anonymous], 1981, 19 AIAA AER M
[3]   Characterization of mixing in a hollow fiber membrane contactor by the iodide-iodate method: Numerical simulations and experiments [J].
Baccar, N. ;
Kieffer, R. ;
Charcosset, C. .
CHEMICAL ENGINEERING JOURNAL, 2009, 148 (2-3) :517-524
[4]  
Baldyga J., 1995, CHEM ENG J, V58, P183, DOI DOI 10.1016/0923-0467(95)02982-6
[5]   Comments on the iodide/iodate method for characterising micromixing [J].
Bourne, John R. .
CHEMICAL ENGINEERING JOURNAL, 2008, 140 (1-3) :638-641
[6]   Mixing and the selectivity of chemical reactions [J].
Bourne, JR .
ORGANIC PROCESS RESEARCH & DEVELOPMENT, 2003, 7 (04) :471-508
[7]   A CONTINUUM METHOD FOR MODELING SURFACE-TENSION [J].
BRACKBILL, JU ;
KOTHE, DB ;
ZEMACH, C .
JOURNAL OF COMPUTATIONAL PHYSICS, 1992, 100 (02) :335-354
[8]   Process intensification: Visual study of liquid maldistribution in rotating packed beds [J].
Burns, JR ;
Ramshaw, C .
CHEMICAL ENGINEERING SCIENCE, 1996, 51 (08) :1347-1352
[9]   Preparation and characterization of zinc sulfide nanoparticles under high-gravity environment [J].
Chen, JF ;
Li, YL ;
Wang, YH ;
Yun, J ;
Cao, DP .
MATERIALS RESEARCH BULLETIN, 2004, 39 (02) :185-194
[10]   Villermaux-Dushman protocol for experimental characterization of micromixers [J].
Commenge, Jean-Marc ;
Falk, Laurent .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2011, 50 (10) :979-990