Transition-metal-doped Fe2O3 nanoparticles for oxygen evolution reaction

被引：47

作者：

Yin, Yichun ^{[1
]}

Zhang, Xiwang ^{[2
]}

Sun, Chenghua ^{[3
]}

机构：

[1] Monash Univ, Sch Chem, ARC Ctr Excellence Electromat Sci, Wellington Rd, Clayton, Vic 3800, Australia

[2] Monash Univ, Dept Chem Engn, Wellington Rd, Clayton, Vic 3800, Australia

[3] Swinbume Univ Technol, Fac Sci Engn & Technol, John St, Hawthorn, Vic 3122, Australia

来源：

PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL | 2018年 / 28卷 / 04期

基金：

澳大利亚研究理事会;

关键词：

Hematite; Metal doping; Water splitting; Oxygen evolution reaction; PHOTO-FENTON REACTION; WATER OXIDATION; PHOTOELECTROCHEMICAL PROPERTIES; SEMICONDUCTOR ELECTRODES; EFFECTIVE DOPANTS; ALPHA-FE2O3; HEMATITE; PERFORMANCE; FILMS; TRANSPARENT;

D O I：

10.1016/j.pnsc.2018.07.005

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

Hematite (alpha-Fe2O3) has been extensively studied as a promising photocatalyst, with the capacity to split water under visible light. To tune its electronic structure and improve the performance for oxygen evolution reaction (OER), high-quality single crystals of alpha-Fe2O3 nanoparticles were synthesized and doped by various transition metals (M = V, Cr, Mn, Zn, Co, Ni, Cu, Nb, Mo, Ti) by a molten-salt flux method. Optical, electronic and catalytic properties of transition-metal-doped alpha-Fe2O3 (TM-doped alpha-Fe2O3) have been systematically investigated. Cobalt has been identified as the best dopant for alpha-Fe2O3, reducing the OER overpotential by 0.16 V with respect to the undoped.

引用

页码：430 / 436

页数：7

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