Optimizing utilization of point source and atmospheric carbon dioxide as a feedstock in electrochemical CO2 reduction

被引:11
作者
Badgett, Alex [1 ]
Feise, Alison [1 ,2 ]
Star, Andrew [3 ]
机构
[1] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA
[2] Univ Toronto, Dept Chem, Toronto, ON M5S 3J6, Canada
[3] Natl Renewable Energy Lab, Chem & Nanosci, 15013 Denver West Pkwy, Golden, CO 80401 USA
关键词
ELECTROLYSIS; TECHNOLOGY; CHALLENGES; CAPTURE; AIR; AG;
D O I
10.1016/j.isci.2022.104270
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The electrochemical reduction of carbon dioxide is a potential pathway for production of fuels and chemicals that uses atmospheric carbon dioxide as a feedstock. Here, we present an analysis of the potential for carbon dioxide from point sources and via direct air capture to be utilized in electrochemical reduction under differentmarket scenarios. We show that developing a network for production of these products at scale requires capture and utilization of significant portions of the carbon dioxide that is currently emitted from large stationary point sources. Because carbon dioxide point sources are spatially and compositionally variable, their use for carbon dioxide reduction depends on electricity prices, capture cost, and location. If the power sector in the United States is decarbonized, carbon dioxide supply decreases significantly, increasing the importance of utilizing other carbon dioxide streams, and increasing the likelihood that direct air capture plays a role in supplying carbon dioxide feedstocks.
引用
收藏
页数:18
相关论文
共 76 条
[1]  
[Anonymous], 2005, Carbon Dioxide Capture and Storage
[2]  
[Anonymous], 2020, Greenhouse Gas Inventory Guidance: Indirect Emissions from Purchased Electricity
[3]  
[Anonymous], 2021, HIFLD Open Data
[4]   Decentralized chemical processes with supercritical fluid technology for sustainable society [J].
Arai, Kunio ;
Smith, Richard L., Jr. ;
Aida, Taku M. .
JOURNAL OF SUPERCRITICAL FLUIDS, 2009, 47 (03) :628-636
[5]   CO2 capture from the industry sector [J].
Bains, Praveen ;
Psarras, Peter ;
Wilcox, Jennifer .
PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 2017, 63 :146-172
[6]   Carbon neutral manufacturing via on-site CO2 recycling [J].
Barecka, Magda H. ;
Ager, Joel W. ;
Lapkin, Alexei A. .
ISCIENCE, 2021, 24 (06)
[7]   Economically viable CO2 electroreduction embedded within ethylene oxide manufacturing [J].
Barecka, Magda H. ;
Ager, Joel W. ;
Lapkin, Alexei A. .
ENERGY & ENVIRONMENTAL SCIENCE, 2021, 14 (03) :1530-1543
[8]  
Becker T., 2021, J BUS ECON STAT, V91, P867, DOI [DOI 10.1007/S11573-020-01019-4, 10.1007/s11573-020-01019-4]
[9]   Julia: A Fresh Approach to Numerical Computing [J].
Bezanson, Jeff ;
Edelman, Alan ;
Karpinski, Stefan ;
Shah, Viral B. .
SIAM REVIEW, 2017, 59 (01) :65-98
[10]   CO2 reduction on gas-diffusion electrodes and why catalytic performance must be assessed at commercially-relevant conditions [J].
Burdyny, Thomas ;
Smith, Wilson A. .
ENERGY & ENVIRONMENTAL SCIENCE, 2019, 12 (05) :1442-1453