Hot Brownian Motion

被引:169
作者
Rings, Daniel [1 ,2 ]
Schachoff, Romy [1 ,2 ]
Selmke, Markus [1 ,2 ]
Cichos, Frank [1 ,2 ]
Kroy, Klaus [1 ,2 ]
机构
[1] Univ Leipzig, Inst Theoret Phys, D-04009 Leipzig, Germany
[2] Univ Leipzig, Inst Expt Phys 1, D-04103 Leipzig, Germany
关键词
PHOTOTHERMAL CORRELATION SPECTROSCOPY; HEAT; NANOPARTICLES; PARTICLES; TRACKING; SYSTEMS; PHYSICS; CELLS;
D O I
10.1103/PhysRevLett.105.090604
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We derive the Markovian description for the nonequilibrium Brownian motion of a heated nanoparticle in a simple solvent with a temperature-dependent viscosity. Our analytical results for the generalized fluctuation-dissipation and Stokes-Einstein relations compare favorably with measurements of laser-heated gold nanoparticles and provide a practical rational basis for emerging photothermal tracer and nanoparticle trapping and tracking techniques.
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页数:4
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共 34 条
[1]   Fluctuations and Response of Nonequilibrium States [J].
Baiesi, Marco ;
Maes, Christian ;
Wynants, Bram .
PHYSICAL REVIEW LETTERS, 2009, 103 (01)
[2]   Photothermal heterodyne imaging of individual nonfluorescent nanoclusters and nanocrystals [J].
Berciaud, S ;
Cognet, L ;
Blab, GA ;
Lounis, B .
PHYSICAL REVIEW LETTERS, 2004, 93 (25)
[3]   Einstein relation generalized to nonequilibrium [J].
Blickle, V. ;
Speck, T. ;
Lutz, C. ;
Seifert, U. ;
Bechinger, C. .
PHYSICAL REVIEW LETTERS, 2007, 98 (21)
[4]   Thermodynamics of a colloidal particle in a time-dependent nonharmonic potential [J].
Blickle, V ;
Speck, T ;
Helden, L ;
Seifert, U ;
Bechinger, C .
PHYSICAL REVIEW LETTERS, 2006, 96 (07)
[5]   Confocal three dimensional tracking of a single nanoparticle with concurrent spectroscopic readouts [J].
Cang, Hu ;
Wong, Chung M. ;
Xu, C. Shan ;
Rizvi, Abbas H. ;
Yang, Haw .
APPLIED PHYSICS LETTERS, 2006, 88 (22)
[6]   Thermophoretic interaction of heat releasing particles [J].
Dolinsky, Y ;
Elperin, T .
JOURNAL OF APPLIED PHYSICS, 2003, 93 (07) :4321-4327
[7]   Relativistic Brownian motion [J].
Dunkel, Joern ;
Haenggi, Peter .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 2009, 471 (01) :1-73
[9]  
Frenkel D, 2006, SCOT GRAD SER, P19
[10]   Brownian motion: a paradigm of soft matter and biological physics [J].
Frey, E ;
Kroy, K .
ANNALEN DER PHYSIK, 2005, 14 (1-3) :20-50