Energy-sensitive imaging detector applied to the dissociative recombination of D2H+

被引：24

作者：

Buhr, H. ^{[1
,2
]}

Mendes, M. B. ^{[2
]}

Novotny, O. ^{[2
]}

Schwalm, D. ^{[1
,2
]}

Berg, M. H. ^{[2
]}

Bing, D. ^{[2
]}

Heber, O. ^{[1
]}

Krantz, C. ^{[2
]}

Orlov, D. A. ^{[2
]}

Rappaport, M. L. ^{[1
]}

Sorg, T. ^{[2
]}

Stuetzel, J. ^{[2
]}

Varju, J. ^{[2
]}

Wolf, A. ^{[2
]}

Zajfman, D. ^{[1
]}

机构：

[1] Weizmann Inst Sci, Fac Phys, IL-76100 Rehovot, Israel

[2] Max Planck Inst Kernphys, D-69121 Heidelberg, Germany

来源：

PHYSICAL REVIEW A | 2010年 / 81卷 / 06期

关键词：

Ions - Kinetic energy - Storage rings - Hydrogen storage - Photodissociation - Electron energy levels;

D O I：

10.1103/PhysRevA.81.062702

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We report on an energy-sensitive imaging detector for studying the fragmentation of polyatomic molecules in the dissociative recombination of fast molecular ions with electrons. The system is based on a large area (10 x 10 cm(2)) position-sensitive, double-sided Si-strip detector with 128 horizontal and 128 vertical strips, whose pulse height information is read out individually. The setup allows us to uniquely identify fragment masses and is thus capable of measuring branching ratios between different fragmentation channels, kinetic energy releases, and breakup geometries as a function of the relative ion-electron energy. The properties of the detection system, which has been installed at the Test Storage Ring (TSR) facility of the Max-Planck Institute for Nuclear Physics in Heidelberg, is illustrated by an investigation of the dissociative recombination of the deuterated triatomic hydrogen cation D2H+. A huge isotope effect is observed when comparing the relative branching ratio between the D-2 + H and the HD + D channel; the ratio 2B(D-2 + H)/B(HD + D), which is measured to be 1.27 +/- 0.05 at relative electron-ion energies around 0 eV, is found to increase to 3.7 +/- 0.5 at similar to 5 eV.

引用

页数：10

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