Externally controlled atom transfer radical polymerization

被引：368
作者：
Pan, Xiangcheng [1 ]
Fantin, Marco [2 ]
Yuan, Fang [1 ]
Matyjaszewski, Krzysztof [2 ]
机构：
[1] Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200433, Peoples R China
[2] Carnegie Mellon Univ, Dept Chem, 4400 5th Ave, Pittsburgh, PA 15213 USA
来源：
CHEMICAL SOCIETY REVIEWS | 2018年 / 47卷 / 14期
基金：
美国国家科学基金会; 中国国家自然科学基金;
关键词：
ELECTROCHEMICALLY MEDIATED ATRP; DISSOCIATIVE ELECTRON-TRANSFER; WELL-DEFINED POLYMERS; FRAGMENTATION CHAIN-TRANSFER; N-BUTYL ACRYLATE; VISIBLE-LIGHT; METHYL-METHACRYLATE; ARGET ATRP; ICAR ATRP; STAR POLYMERS;
D O I：
10.1039/c8cs00259b
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Spatial and temporal regulations of ATRP by external stimuli are presented. Various ATRP techniques, eATRP, photoATRP, and mechanoATRP, are controlled by electrical current, light, and mechanical forces, respectively. Conversely, ARGET and SARA ATRP are controlled by chemical reducing agents. ICAR ATRP is a thermally regulated process through decomposition of a radical initiator. The aim of this review is to highlight the use of external regulations in ATRP and to summarize the state-of-the-art and future perspectives, focusing on mechanistic aspects, synthetic procedures, preparation of polymers with complex architectures and functional materials, and their applications.
引用
收藏
页码：5457 / 5490
页数：34
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