Enrichment of residual carbon from coal gasification fine slag in an inflatable-inclined liquid-solid fluidized bed

被引:28
作者
Lv, Bo [1 ,2 ,3 ]
Zhao, Zeya [1 ]
Dong, Bobing [1 ,2 ]
Deng, Xiaowei [1 ,2 ,3 ,4 ]
Fang, Chaojun [1 ,2 ]
Zhang, Bo [5 ]
机构
[1] Henan Polytech Univ, Coll Chem & Chem Engn, Jiaozuo 454000, Henan, Peoples R China
[2] State Key Lab Mineral Proc, Beijing 100260, Peoples R China
[3] Henan Polytech Univ, Henan Key Lab Green & Efficient Min & Comprehens, Jiaozuo 454000, Henan, Peoples R China
[4] Henan Polytech Univ, Collaborat Innovat Ctr Coal Work Safety & Clean H, Jiaozuo 454000, Henan, Peoples R China
[5] China Univ Min & Technol, Key Lab Coal Proc & Efficient Utilizat, Minist Educ, Xuzhou 221116, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Liquid-solid fluidized bed; Gasification fine slag; Concentrate product; Residual carbon; Combustion performance; UNBURNED CARBON; FLOTATION; PARTICLES;
D O I
10.1016/j.jclepro.2022.131132
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The recovery and utilization of the fine slag obtained from coal gasification is of great significance to reduce environmental pollution and improve resource utilization. An inflatable-inclined liquid-solid fluidized bed was used to enrich and recover residual carbon from coal gasification fine slag, and the separation principles and influencing factors were investigated by numerical simulation and experiments. The results showed that light and heavy particles were initially separated by increasing the water flow in the vertical section of the bed when the slag entered the liquid-solid fluidized bed. Subsequently, a secondary air flow further separated light par-ticles from heavy ones on the inclined section of the bed, which strengthened the overall separation effect of the liquid-solid fluidized bed for gasification fine slag. During the separation process, the loss-on-ignition and re-sidual carbon recovery percentage of the concentrate first increased and then decreased; they increased with the increase in rising water velocity (and secondary air velocity) but decreased with the increase in feed quantity. The influence of these factors on the loss-on-ignition and residual carbon recovery percentage of the concentrate was as follows: water velocity (v(w)) > feed quantity (m) > secondary air velocity (v(f)). Under suitable operating conditions (m = 200 g, v(w) = 0.042 m/s, v(f )= 2.12 m/s), the loss-on-ignition of the concentrate reached 66.38%, which represents a high carbon content, thereby indicating that the liquid-solid fluidized bed efficiently enriched the residual carbon in the fine slag. According to loss-on-ignition of the concentrate and product characteristics through scanning electron microscope and thermogravimetric analysis, the concentrate has a high carbon con -tent (loss-on-ignition of 66.38%) and high reactivity, which can be used as fuel. The findings of this study will provide a theoretical and technical basis for the resource utilization of coal gasification fine slag.
引用
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页数:12
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