Selective assembly of magnetic nano-antenna for electromagnetic dissipation

被引:15
作者
Fang, Jiefeng [1 ]
Lv, Hualiang [1 ]
Zhao, Biao [1 ]
Liu, Zhengwang [1 ]
Li, Xiaohui [1 ]
Xu, Chunyang [1 ]
Zhang, Ruixuan [1 ]
Zhang, Huibin [1 ]
Liu, Xianhu [2 ]
Zhang, Xuefeng [3 ]
Wang, Min [1 ]
Che, Renchao [1 ,4 ]
机构
[1] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Dept Mat Sci, Lab Adv Mat, Shanghai 200438, Peoples R China
[2] Zhengzhou Univ, Minist Educ, Key Lab Mat Proc & Mold, Zhengzhou 450002, Peoples R China
[3] Hangzhou Dianzi Univ, Coll Mat & Environm Engn, Inst Adv Magnet Mat, Hangzhou 310012, Peoples R China
[4] Zhejiang Lab, Joint Res Ctr Computat Mat, Hangzhou 311100, Peoples R China
基金
中国国家自然科学基金;
关键词
ENHANCED MICROWAVE-ABSORPTION; FACILE SYNTHESIS; AT-C; COMPOSITES; NANOPARTICLES; NANOFIBERS;
D O I
10.1039/d2ta02186b
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Assembly of multiple-component composites into a beneficial multi-shell structure has been demonstrated as an efficient strategy to induce wideband electromagnetic (EM) attenuation in principle. However, structural engineering with selective components remains challenging, hindering the development of high-performance EM absorbers. Herein, a distinctive structure of large-scale magnetic particle-decorated multi-branch Fe@SiO2@Fe is proposed, obtained via an anisotropic magnetic loading strategy to achieve broadband microwave attenuation performance. Adjusting the interaction force equilibrium between magnetic particles and silica, a uniform coating layer composed of bulky magnetic particles on a 3D template is fabricated. The effective microwave bandwidth is broadened by the enhanced magnetic response range with multi-scale magnetic couplings and remarkable hierarchical interfacial polarization in our highly symmetrical structure, reaching 11.5 GHz at a thickness of 2.5 mm. Our component and structural modulation provides a strategy for achieving ultra-broadband EM absorption by anisotropic design.
引用
收藏
页码:10909 / 10915
页数:7
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