Transparent, smooth, and sustainable cellulose-derived conductive film applied for the flexible electronic device

被引:23
作者
Liu, Xi [1 ,2 ]
Xiao, Wei [1 ,2 ]
Tao, Tao [1 ,2 ]
Yang, Jiawei [1 ,2 ]
Li, Huixin [1 ,2 ]
Chen, Qunfeng [1 ,2 ]
Huang, Liulian [1 ,2 ]
Ni, Yonghao [1 ,3 ]
Chen, Lihui [1 ,2 ]
Ouyang, Xinhua [1 ,2 ]
Zhu, Xuhai [4 ,5 ]
Li, Jianguo [1 ,2 ]
机构
[1] Fujian Agr & Forestry Univ, Coll Mat Engn, Fuzhou 350002, Fujian, Peoples R China
[2] Natl Forestry & Grassland Adm Key Lab Plant Fiber, Fuzhou, Peoples R China
[3] Univ New Brunswick, Dept Chem Engn, Limerick Pulp & Paper Ctr, Fredericton, NB E3B 5A3, Canada
[4] Aalto Univ, Dept Bioprod & Biosyst, Sch Chem Engn, Vuorimiehentie 1, Espoo 02150, Finland
[5] Chinese Acad Sci, State Key Lab Catalysis, Dalian Natl Lab Clean Energy, Dalian Inst Chem Phys, Dalian 110623, Liaoning, Peoples R China
基金
中国国家自然科学基金;
关键词
Cellulose; Conductive film; ZnO buffer layer; Flexible electronic device; CARBON NANOTUBE; COMPOSITE FILMS; THIN; LIGNIN;
D O I
10.1016/j.carbpol.2021.117820
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
A high-performance flexible conductive substrate is one of the key components for developing promising wearable devices. Concerning this, a sustainable, flexible, transparent, and conductive cellulose/ZnO/AZO (CZA) film was developed in this study. The cellulose was used as the transparent substrate. The added AZO was as the conductive layer and ZnO functioned as an interface buffer layer. Results showed that the interface buffer layer of ZnO effectively alleviated the intrinsic incompatibility of organic cellulose and inorganic AZO, resulting in the improvement of the performance of CZA film. In compared with the controlled cellulose/AZO (CA) film with 365 ?/sq sheet resistance and 87% transmittance, this CZA film featured a low conductive sheet resistance of 115 ?/sq and high transmittance of 89%, as well as low roughness of 1.85 nm Moreover, the existence of conducive ZnO buffer layer enabled the conductivity of CZA film to be stable under the bending treatment. Herein, a flexible electronic device was successfully prepared with the biomass materials, which would be available by a roll-to-roll production process.
引用
收藏
页数:7
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