Catalytic partial oxidation (CPOX) of natural gas and renewable hydrocarbons/oxygenated hydrocarbons-A review

被引：53
作者：
Ma, Ruoshui [1 ,2 ]
Xu, Bang [3 ]
Zhang, Xiao [1 ,2 ]
机构：
[1] Washington State Univ, Voiland Sch Chem Engn & Bioengn, 2710 Crimson Way, Richland, WA 99354 USA
[2] Pacific Northwest Natl Lab, 2710 Crimson Way, Richland, WA 99354 USA
[3] Dason Technol, 3100 George Washington Way,S108, Richland, WA 99354 USA
来源：
CATALYSIS TODAY | 2019年 / 338卷
关键词：
Partial oxidation; Natural Gas; Reforming; Catalysis; Renewable; PEROVSKITE-TYPE OXIDES; METHANE PARTIAL OXIDATION; FLUIDIZED-BED REACTOR; HYDROGEN-PRODUCTION; OXYGEN-CARRIER; CARBON-MONOXIDE; SELECTIVE OXIDATION; FUEL-CELLS; BIO-OIL; BIOMASS GASIFICATION;
D O I：
10.1016/j.cattod.2019.06.025
中图分类号：
O69 [应用化学];
学科分类号：
081704 ;
摘要：
Catalytic partial oxidation (CPOX) is one of the most promising technologies for converting natural gas for fuel and chemicals synthesis. CPOX has been gaining increasing attention for conversion of natural gas to ideal syngas mixtures for fuel production. The urgency and importance of this endeavour has been increasingly recognized in the last few years due to the exploration of shale gas and flare gas. However, the information regarding the progress of industrial implementation of this technology is scarce. This review presents recent advances of CPOX techniques from bench to pilot scale and a comparison of its energy efficiency, carbon conversion efficiency, and operating costs with parallel technologies including steam reforming (SMR), autothermal reforming (ATR), and partial oxidation (POX). The potential applications and perspective of CPOX for long chain hydrocarbon and renewable hydrocarbon/oxygenated hydrocarbons conversion to new platform chemical and materials is also discussed.
引用
收藏
页码：18 / 30
页数：13
相关论文
共 248 条
  • [61] Nanoscale Cu supported catalysts in the partial oxidation of cyclohexane with molecular oxygen
    Evangelisti, Claudio
    Vitulli, Giovanni
    Schiavi, Eleonora
    Vitulli, Maria
    Bertozzi, Sergio
    Salvadori, Piero
    Bertinetti, Luca
    Martra, Gianmario
    [J]. CATALYSIS LETTERS, 2007, 116 (1-2) : 57 - 62
  • [62] Farina G., 1992, HYDROCARBON PROCESS, V71
  • [63] Environmental catalysis into the 21st century
    Farrauto, RJ
    Heck, RM
    [J]. CATALYSIS TODAY, 2000, 55 (1-2) : 179 - 187
  • [64] Partial oxidation of methane to synthesis gas: Elimination of gas phase oxygen
    Fathi, M
    Bjorgum, E
    Viig, T
    Rokstad, OA
    [J]. CATALYSIS TODAY, 2000, 63 (2-4) : 489 - 497
  • [65] Effect of base additives on the selective hydrogenolysis of glycerol over Ru/TiO2 catalyst
    Feng, Jian
    Wang, Jinbo
    Zhou, Yafen
    Fu, Haiyan
    Chen, Hua
    Li, Xianjun
    [J]. CHEMISTRY LETTERS, 2007, 36 (10) : 1274 - 1275
  • [66] Fleisch T.H., 2002, J NAT GAS CHEM, V11, P1, DOI DOI 10.1016/S0140-6701(03)91770-X
  • [67] Selective catalytic oxidation of glyceric acid to tartronic and hydroxypyruvic acids
    Fordham, P
    Besson, M
    Gallezot, P
    [J]. APPLIED CATALYSIS A-GENERAL, 1995, 133 (02) : L179 - L184
  • [68] Theoretical investigation of the system SnOx/Sn for the thermochemical storage of solar energy
    Forster, M
    [J]. ENERGY, 2004, 29 (5-6) : 789 - 799
  • [69] DIRECT CATALYTIC-OXIDATION OF METHANE TO METHANOL - A REVIEW
    FOSTER, NR
    [J]. APPLIED CATALYSIS, 1985, 19 (01): : 1 - 11
  • [70] Biotransformation of glycerol to dihydroxyacetone by recombinant Gluconobacter oxydans DSM 2343
    Gaetgens, Cornelia
    Degner, Ursula
    Bringer-Meyer, Stephanie
    Herrmann, Ute
    [J]. APPLIED MICROBIOLOGY AND BIOTECHNOLOGY, 2007, 76 (03) : 553 - 559
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