Photocurrent Induced by Nonradiative Energy Transfer from Nanocrystal Quantum Dots to Adjacent Silicon Nanowire Conducting Channels: Toward a New Solar Cell Paradigm

被引:73
|
作者
Lu, Siyuan [1 ]
Lingley, Zachary [2 ]
Asano, Tetsuya [2 ]
Harris, Daniel [2 ]
Barwicz, Tymon [3 ]
Guha, Supratik [3 ]
Madhukar, Anupam [1 ,2 ]
机构
[1] Univ So Calif, Dept Phys, Los Angeles, CA 90089 USA
[2] Univ So Calif, Mork Family Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA
[3] IBM Corp, JT Watson Res Ctr, Yorktown Hts, NY 10598 USA
关键词
EXCITATION;
D O I
10.1021/nl903104k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report the observation of photocurrent in silicon nanowires induced by nonradiative resonant energy transfer (NRET) from adjacent layers of lead sulfide nanocrystal quantum dots using time-resolved photocurrent measurements. This demonstration supports the feasibility of a new solar cell paradigm (Lu, S.; Madhukar, A. Nano Lett. 2007, 7, 3443-3451) that exploits NRET between efficient photon absorbers and adjacent nanowire/quantum well high-mobility charge transport channels and could offer a viable alternative to the limitations of carrier transport and collection faced by excitonic solar cells.
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收藏
页码:4548 / 4552
页数:5
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