Fabrication and antifouling behaviour of a carbon nanotube membrane

被引:68
作者
Ihsanullah [1 ]
Al Amer, Adnan M. [1 ]
Laoui, Tahar [2 ]
Abbas, Aamir [1 ]
Al-Aqeeli, Nasser [2 ]
Patel, Faheemuddin [2 ]
Khraisheh, Marwan [3 ]
Atieh, Muataz Ali [3 ,4 ]
Hilal, Nidal [3 ,5 ]
机构
[1] King Fahd Univ Petr & Minerals, Dept Chem Engn, Dhahran 31261, Saudi Arabia
[2] King Fahd Univ Petr & Minerals, Dept Mech Engn, Dhahran 31261, Saudi Arabia
[3] Qatar Fdn, Qatar Environm & Energy Res Inst, Doha, Qatar
[4] Hamad Bin Khalifa Univ, Qatar Fdn, Coll Sci & Engn, Doha, Qatar
[5] Swansea Univ, Coll Engn, Ctr Water Adv Technol & Environm Res CWATER, Swansea SA2 8PP, W Glam, Wales
关键词
Membrane; Iron oxide; Water treatment; Carbon nanotubes; Sodium alginate; MECHANICAL-PROPERTIES; AQUEOUS-SOLUTION; ADSORPTION; ULTRAFILTRATION; WATER; COMPOSITE; DESALINATION; ALGINATE; RECOVERY; NI(II);
D O I
10.1016/j.matdes.2015.10.018
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In this work, a novel approach is used to synthesize an iron oxide doped carbon nanotube (CNT) membrane, with the goal of fully utilizing the unique properties of CNTs. No binder is used for the synthesis of the membrane; instead, iron oxide particles serve as a binding agent for holding the CNTs together after sintering at high temperature. The produced membrane exhibited a high water flux and strong fouling resistance. In the first step, CNTs were impregnated with various loadings of iron oxide (1, 10, 20, 30 and 50%) via wet chemistry techniques. Impregnated CNTs were then compacted at 200 MPa and sintered at 1350 degrees C for 5 h to form a compact disc. The membranes were analysed by measuring their porosity, contact angle, diametrical compression test and water flux. The flux of pure water was observed to increase with an increase in iron oxide content The permeate flux and rejection rate of sodium alginate (SA) were determined to predict the antifouling behaviour of the membrane. A maximum removal of 90 and 88% of SA was achieved for membranes with a 10 and 1% iron oxide content, respectively, after 3 h. A minor decline in the permeate flux was observed for all membranes after 4 h of operation. (C) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:549 / 558
页数:10
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