Ultrafast relaxation of hot phonons in graphene-hBN heterostructures

被引:37
作者
Golla, Dheeraj [1 ]
Brasington, Alexandra [1 ]
LeRoy, Brian J. [1 ]
Sandhu, Arvinder [1 ]
机构
[1] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA
基金
美国国家科学基金会;
关键词
ELECTRON-TRANSPORT; DYNAMICS; NANOTUBES;
D O I
10.1063/1.4982738
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Fast carrier cooling is important for high power graphene based devices. Strongly coupled optical phonons play a major role in the relaxation of photo-excited carriers in graphene. Heterostructures of graphene and hexagonal boron nitride (hBN) have shown exceptional mobility and high saturation current, which makes them ideal for applications, but the effect of the hBN substrate on carrier cooling mechanisms is not understood. We track the cooling of hot photo-excited carriers in graphene-hBN heterostructures using ultrafast pump-probe spectroscopy. We find that the carriers cool down four times faster in the case of graphene on hBN than on a silicon oxide substrate thus overcoming the hot phonon bottleneck that plagues cooling in graphene devices. (C) 2017 Author(s).
引用
收藏
页数:6
相关论文
共 39 条
[1]   Optical Probing of the Electronic Interaction between Graphene and Hexagonal Boron Nitride [J].
Ahn, Gwanghyun ;
Kim, Hye Ri ;
Ko, Taeg Yeoung ;
Choi, Kyoungjun ;
Watanabe, Kenji ;
Taniguchi, Takashi ;
Hong, Byung Hee ;
Ryu, Sunmin .
ACS NANO, 2013, 7 (02) :1533-1541
[2]   Inelastic carrier lifetime in a coupled graphene/electron-phonon system: Role of plasmon-phonon coupling [J].
Ahn, Seongjin ;
Hwang, E. H. ;
Min, Hongki .
PHYSICAL REVIEW B, 2014, 90 (24)
[3]   Electronic Cooling in Graphene [J].
Bistritzer, R. ;
MacDonald, A. H. .
PHYSICAL REVIEW LETTERS, 2009, 102 (20)
[4]   Phonon anharmonicities in graphite and graphene [J].
Bonini, Nicola ;
Lazzeri, Michele ;
Marzari, Nicola ;
Mauri, Francesco .
PHYSICAL REVIEW LETTERS, 2007, 99 (17)
[5]   Thermal interface conductance across a graphene/hexagonal boron nitride heterojunction [J].
Chen, Chun-Chung ;
Li, Zhen ;
Shi, Li ;
Cronin, Stephen B. .
APPLIED PHYSICS LETTERS, 2014, 104 (08)
[6]   Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor [J].
Das, A. ;
Pisana, S. ;
Chakraborty, B. ;
Piscanec, S. ;
Saha, S. K. ;
Waghmare, U. V. ;
Novoselov, K. S. ;
Krishnamurthy, H. R. ;
Geim, A. K. ;
Ferrari, A. C. ;
Sood, A. K. .
NATURE NANOTECHNOLOGY, 2008, 3 (04) :210-215
[7]   Measurement of ultrafast carrier dynamics in epitaxial graphene [J].
Dawlaty, Jahan M. ;
Shivaraman, Shriram ;
Chandrashekhar, Mvs ;
Rana, Farhan ;
Spencer, Michael G. .
APPLIED PHYSICS LETTERS, 2008, 92 (04)
[8]   Boron nitride substrates for high-quality graphene electronics [J].
Dean, C. R. ;
Young, A. F. ;
Meric, I. ;
Lee, C. ;
Wang, L. ;
Sorgenfrei, S. ;
Watanabe, K. ;
Taniguchi, T. ;
Kim, P. ;
Shepard, K. L. ;
Hone, J. .
NATURE NANOTECHNOLOGY, 2010, 5 (10) :722-726
[9]   High thermoelectricpower factor in graphene/hBN devices [J].
Duan, Junxi ;
Wang, Xiaoming ;
Lai, Xinyuan ;
Li, Guohong ;
Watanabe, Kenji ;
Taniguchi, Takashi ;
Zebarjadi, Mona ;
Andrei, Eva Y. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2016, 113 (50) :14272-14276
[10]  
Edgar J. H., 1994, ENG TECHNOLOGY