Half- and full-integer power law for distance fluctuations: Langevin dynamics in one- and two-dimensional systems

被引:1
作者
Chen, Wei- Chen [1 ]
Tang, Jau [1 ]
机构
[1] CALTECH, Ctr Ultrafast Sci & Technol, Noyes Lab 127 72, Pasadena, CA 91125 USA
基金
美国国家科学基金会;
关键词
power laws; Langevin dynamics; single molecule; Rouse model;
D O I
10.1016/j.chemphys.2006.10.012
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Langevin dynamics of one- and two-dimensional systems with the nearest neighbor couplings is examined to derive the autocorrelation function (ACF) of the distance fluctuations. Understanding of the dynamics of pairwise distance correlation is essential in the studies using single-molecule spectroscopy. For both 1-D cases of an open chain and a closed loop, a power law of t-(1/2), t(-3/2) and t(-5/2) for the ACF are obtained, and for 2-D systems of a sheet and a tube, a power law of t(-1), t(-2) and t(-3) are found. The different exponent of the power law is shown to depend on the location of the pairwise beads and their topography. (c) 2006 Elsevier B.V. All rights reserved.
引用
收藏
页码:245 / 253
页数:9
相关论文
共 40 条
[1]   Langevin modes analysis of myoglobin [J].
Ansari, A .
JOURNAL OF CHEMICAL PHYSICS, 1999, 110 (03) :1774-1780
[2]   Diffusion-assisted long-range reaction between the ends of a polymer: Effective sink approximation [J].
Barzykin, AV ;
Seki, K ;
Tachiya, M .
JOURNAL OF CHEMICAL PHYSICS, 2002, 117 (03) :1377-1384
[3]   Irreversible bimolecular reactions of Langevin particles [J].
Bicout, DJ ;
Berezhkovskii, AM ;
Szabo, A .
JOURNAL OF CHEMICAL PHYSICS, 2001, 114 (05) :2293-2303
[4]   TEMPERATURE-DEPENDENCE OF PHASE BREAKING IN BALLISTIC QUANTUM DOTS [J].
CLARKE, RM ;
CHAN, IH ;
MARCUS, CM ;
DURUOZ, CI ;
HARRIS, JS ;
CAMPMAN, K ;
GOSSARD, AC .
PHYSICAL REVIEW B, 1995, 52 (04) :2656-2659
[5]   Harmonic behavior of trehalose-coated carbon-monoxy-myoglobin at high temperature [J].
Cordone, L ;
Ferrand, M ;
Vitrano, E ;
Zaccai, G .
BIOPHYSICAL JOURNAL, 1999, 76 (02) :1043-1047
[6]   Multiple time scale dynamics of distance fluctuations in a semiflexible polymer: A one-dimensional generalized Langevin equation treatment [J].
Debnath, P ;
Min, W ;
Xie, S ;
Cherayil, BJ .
JOURNAL OF CHEMICAL PHYSICS, 2005, 123 (20)
[7]  
DEGENNES PG, 1985, SCALING CONCEPTS POL
[8]  
Doi M., 1988, THEORY POLYM DYNAMIC
[9]   The hydrodynamics of DNA electrophoretic stretch and relaxation in a polymer solution [J].
Ferree, S ;
Blanch, HW .
BIOPHYSICAL JOURNAL, 2004, 87 (01) :468-475
[10]  
Gradshteyn I. S., 1980, Gos. Izd-vo Fiz.-Mat. Literatury