Rational Optimization of Benzo[2,1-b;3,4-b′]dithilophene-Containing Polymers for Organic Field-Effect Transistors

被引:72
|
作者
Rieger, Ralph [1 ]
Beckmann, Dirk [1 ]
Pisula, Wojciech [1 ]
Steffen, Werner [1 ]
Kastler, Marcel [1 ]
Muellen, Klaus [1 ]
机构
[1] Max Planck Inst Polymer Res, D-55128 Mainz, Germany
关键词
THIN-FILM TRANSISTORS; CHARGE-TRANSPORT PROPERTIES; POLYTHIOPHENE; SEMICONDUCTORS; MOBILITY; NANOPARTICLES; MORPHOLOGY;
D O I
10.1002/adma.200901286
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The rational structure optimization of a polythiophene containing benzo[2,1b;3,4-b']dithiophene on the molecular level leads to a polymer that is easily synthesized and processed. Fabricated on a flexible substrate, the polymer shows excellent device characteristics, good reproducibility, and charge-carrier mobilities up to 0.5 cm(2) V-1 s(-1) without annealing.
引用
收藏
页码:83 / +
页数:5
相关论文
共 50 条
  • [21] Experimental and computational studies of 4H-cyclopenta[2,1-b:3,4-b′]dithiophen-4-one (CPDTO)-oligomers
    Zhang, Cheng
    Sun, Jianyuan
    Qiao, Qiquan
    Li, Jing
    POLYMER, 2014, 55 (18) : 4677 - 4683
  • [22] Diseleno[3,2-b:2′,3′-d]selenophene-Containing High-Mobility Conjugated Polymer for Organic Field-Effect Transistors
    Jang, Soo-Young
    Kim, In-Bok
    Kang, Minji
    Fei, Zuping
    Jung, Eunhwan
    McCarthy-Ward, Thomas
    Shaw, Jessica
    Lim, Dae-Hee
    Kim, Yeon-Ju
    Mathur, Sanjay
    Heeney, Martin
    Kim, Dong-Yu
    ADVANCED SCIENCE, 2019, 6 (13)
  • [23] Effect of extended alkyl auxiliary groups on optical and electronic properties of Benzo[2,1-b:3,4-b′:5,6-c"]trithiophene derivatives at bulk level: a first-principles study
    Chaudhry, Aijaz Rasool
    Ul Haq, Bakhtiar
    Muhammad, Shabbir
    Laref, A.
    Hussain, Arshad
    Al-Sehemi, Abdullah G.
    MATERIALS RESEARCH EXPRESS, 2019, 6 (09):
  • [24] Thieno[3,2-b]pyrrole and Benzo[c][1,2,5]thiadiazole Donor-Acceptor Semiconductors for Organic Field-Effect Transistors
    Gunawardhana, Ruwan
    Bulumulla, Chandima
    Gamage, Prabhath L.
    Timmerman, Adam J.
    Udamulle, Chinthaka M.
    Biewer, Michael C.
    Stefan, Mihaela C.
    ACS OMEGA, 2019, 4 (22): : 19676 - 19682
  • [25] Synthesis and characterization of benzo[b]thieno[2,3-d]thiophene (BTT) derivatives as solution-processable organic semiconductors for organic field-effect transistors
    Lee, Yongchul
    Ryu, Soomin
    Choi, Eunjin
    Ho, Dongil
    Earmme, Taeshik
    Kim, Choongik
    Seo, SungYong
    SYNTHETIC METALS, 2021, 282 (282)
  • [26] Vinylene and benzo[c][1,2,5]thiadiazole: effect of the π-spacer unit on the properties of bis(2-oxoindolin-3-ylidene)-benzodifuran-dione containing polymers for n-channel organic field-effect transistors
    Thu Trang Do
    Patil, Basanagouda B.
    Singh, Samarendra P.
    Yambem, Soniya D.
    Feron, Krishna
    Ostrikov, Kostya
    Bell, John M.
    Sonar, Prashant
    RSC ADVANCES, 2018, 8 (68): : 38919 - 38928
  • [27] The structure-property relationship study of electron-deficient dihydroindeno[2,1-b]fluorene derivatives for n-type organic field effect transistors
    Romain, Maxime
    Chevrier, Michele
    Bebiche, Sarah
    Mohammed-Brahim, Tayeb
    Rault-Berthelot, Joelle
    Jacques, Emmanuel
    Poriel, Cyril
    JOURNAL OF MATERIALS CHEMISTRY C, 2015, 3 (22) : 5742 - 5753
  • [28] Near Infrared Absorbing Soluble Poly(cyclopenta[2,1-b:3,4-b′]dithiophen-4-one)vinylene Polymers Exhibiting High Hole and Electron Mobilities in Ambient Air
    Fei, Zhuping
    Gao, Xiang
    Smith, Jeremy
    Pattanasattayavong, Pichaya
    Domingo, Ester Buchaca
    Stingelin, Natalie
    Watkins, Scott E.
    Anthopoulos, Thomas D.
    Kline, R. Joseph
    Heeney, Martin
    CHEMISTRY OF MATERIALS, 2013, 25 (01) : 59 - 68
  • [29] Synthesis and characterization of soluble indolo[3,2-b]carbazole derivatives for organic field-effect transistors
    Boudreault, Pierre-Luc T.
    Virkar, Ajay A.
    Bao, Zhenan
    Leclerc, Mario
    ORGANIC ELECTRONICS, 2010, 11 (10) : 1649 - 1659
  • [30] 4H-Cyclopenta[2,1-b:3,4-b′]Dithiophen-4-One (CPDTO) Homopolymer with Side Chains on Every Other CPDTO
    Sun, Jianyuan
    Venkatesan, Swaminathan
    Dubey, Ashish
    Qiao, Qiquan
    Zhang, Cheng
    JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY, 2017, 55 (06) : 1077 - 1085