Radiative absorption enhancement from coatings on black carbon aerosols

被引：98

作者：

Cui, Xinjuan ^{[1
]}

Wang, Xinfeng ^{[1
]}

Yang, Lingxiao ^{[1
]}

Chen, Bing ^{[1
]}

Chen, Jianmin ^{[1
]}

Andersson, August ^{[2
,3
]}

Gustafsson, Orjan ^{[2
,3
]}

机构：

[1] Shandong Univ, Environm Res Inst, Sch Environm Sci & Engn, Jinan 250100, Peoples R China

[2] Stockholm Univ, Dept Environm Sci & Analyt Chem ACES, SE-10691 Stockholm, Sweden

[3] Stockholm Univ, Bolin Ctr Climate Res, SE-10691 Stockholm, Sweden

来源：

SCIENCE OF THE TOTAL ENVIRONMENT | 2016年 / 551卷

基金：

中国国家自然科学基金;

关键词：

Black carbon; Aerosol mixing states; Lensing effect; Radiative absorption; China; OPTICAL-PROPERTIES; LIGHT-ABSORPTION; ORGANIC-CARBON; BROWN CARBON; MIXING STATE; ELEMENTAL CARBON; SOOT; ASIA; TEMPERATURE; MORPHOLOGY;

D O I：

10.1016/j.scitotenv.2016.02.026

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The radiative absorption enhancement of ambient black carbon (BC), by light-refractive coatings of atmospheric aerosols, constitutes a large uncertainty in estimates of climate forcing. The direct measurements of radiative absorption enhancement require the experimentally-removing the coating materials in ambient BC-containing aerosols, which remains a challenge. Here, the absorption enhancement of the BC core by non-absorbing aerosol coatings was quantified using a two-step removal of both inorganic and organic matter coatings of ambient aerosols. The mass absorption cross-section (MAC) of decoated/pure atmospheric BC aerosols of 4.4 +/- 0.8 m(2)g(-1) was enhanced to 9.6 +/- 1.8 m(2)g(-1) at 678-nm wavelength for ambiently-coated BC aerosols at a rural Northern China site. The enhancement of MAC (E-MAC) rises from 1.4 +/- 0.3 in fresh combustion emissions to similar to 3 for aged ambient China aerosols. The three-week high-intensity campaign observed an average E-MAC of 2.25 +/- 0.55, and sulfates were primary drivers of the enhanced BC absorption. (C) 2016 Elsevier B.V. All rights reserved.

引用

页码：51 / 56

页数：6

共 36 条

[1] Effect of intrinsic organic carbon on the optical properties of fresh diesel soot [J].

Adler, Gabriella ;

Riziq, Ali Abo ;

Erlick, Carynelisa ;

Rudich, Yinon .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2010, 107 (15) :6699-6704

[2] Recent Northern Hemisphere tropical expansion primarily driven by black carbon and tropospheric ozone [J].

Allen, Robert J. ;

Sherwood, Steven C. ;

Norris, Joel R. ;

Zender, Charles S. .

NATURE, 2012, 485 (7398) :350-U93

[3] Bounding the role of black carbon in the climate system: A scientific assessment [J].

Bond, T. C. ;

Doherty, S. J. ;

Fahey, D. W. ;

Forster, P. M. ;

Berntsen, T. ;

DeAngelo, B. J. ;

Flanner, M. G. ;

Ghan, S. ;

Kaercher, B. ;

Koch, D. ;

Kinne, S. ;

Kondo, Y. ;

Quinn, P. K. ;

Sarofim, M. C. ;

Schultz, M. G. ;

Schulz, M. ;

Venkataraman, C. ;

Zhang, H. ;

Zhang, S. ;

Bellouin, N. ;

Guttikunda, S. K. ;

Hopke, P. K. ;

Jacobson, M. Z. ;

Kaiser, J. W. ;

Klimont, Z. ;

Lohmann, U. ;

Schwarz, J. P. ;

Shindell, D. ;

Storelvmo, T. ;

Warren, S. G. ;

Zender, C. S. .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2013, 118 (11) :5380-5552

[4] Limitations in the enhancement of visible light absorption due to mixing state [J].

Bond, Tami C. ;

Habib, Gazala ;

Bergstrom, Robert W. .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2006, 111 (D20)

[5] Light absorption by carbonaceous particles: An investigative review [J].

Bond, TC ;

Bergstrom, RW .

AEROSOL SCIENCE AND TECHNOLOGY, 2006, 40 (01) :27-67

[6] Radiative Absorption Enhancements Due to the Mixing State of Atmospheric Black Carbon [J].

Cappa, Christopher D. ;

Onasch, Timothy B. ;

Massoli, Paola ;

Worsnop, Douglas R. ;

Bates, Timothy S. ;

Cross, Eben S. ;

Davidovits, Paul ;

Hakala, Jani ;

Hayden, Katherine L. ;

Jobson, B. Tom ;

Kolesar, Katheryn R. ;

Lack, Daniel A. ;

Lerner, Brian M. ;

Li, Shao-Meng ;

Mellon, Daniel ;

Nuaaman, Ibraheem ;

Olfert, Jason S. ;

Petaja, Tuukka ;

Quinn, Patricia K. ;

Song, Chen ;

Subramanian, R. ;

Williams, Eric J. ;

Zaveri, Rahul A. .

SCIENCE, 2012, 337 (6098) :1078-1081

[7] Source Forensics of Black Carbon Aerosols from China [J].

Chen, Bing ;

Andersson, August ;

Lee, Meehye ;

Kirillova, Elena N. ;

Xiao, Qianfen ;

Krusa, Martin ;

Shi, Meinan ;

Hu, Ke ;

Lu, Zifeng ;

Streets, David G. ;

Du, Ke ;

Gustafsson, Orjan .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2013, 47 (16) :9102-9108

[8] Mass absorption efficiency of elemental carbon and water-soluble organic carbon in Beijing, China [J].

Cheng, Y. ;

He, K-B ;

Zheng, M. ;

Duan, F-K ;

Du, Z-Y ;

Ma, Y-L ;

Tan, J-H ;

Yang, F-M ;

Liu, J-M ;

Zhang, X-L ;

Weber, R. J. ;

Bergin, M. H. ;

Russell, A. G. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (22) :11497-11510

[9] Climate response of direct radiative forcing of anthropogenic black carbon [J].

Chung, SH ;

Seinfeld, JH .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D11) :1-25

[10] Insights into summertime haze pollution events over Shanghai based on online water-soluble ionic composition of aerosols [J].

Du, Huanhuan ;

Kong, Lingdong ;

Cheng, Tiantao ;

Chen, Jianmin ;

Du, Jianfei ;

Li, Ling ;

Xia, Xiangao ;

Leng, Chunpeng ;

Huang, Guanghan .

ATMOSPHERIC ENVIRONMENT, 2011, 45 (29) :5131-5137

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