Al3+ doping effects and high-field phase diagram of La0.5Sr0.5Mn1-xAlxO3

被引:6
作者
Shang, C. [1 ,2 ]
Xia, Z. C. [1 ]
Wei, M. [1 ,2 ]
Jin, Z. [1 ,2 ]
Chen, B. R. [1 ,2 ]
Shi, L. R. [1 ,2 ]
Ouyang, Z. W. [1 ]
Huang, S. [1 ,2 ]
Xiao, G. L. [1 ,2 ]
机构
[1] Huazhong Univ Sci & Technol, Wuhan Natl High Magnet Field Ctr, Wuhan 430074, Peoples R China
[2] Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
基金
中国国家自然科学基金;
关键词
manganites; phase transition; doping; pulsed high magnetic field; INSULATOR-METAL TRANSITION; MAGNETIC-FIELD; TRANSPORT-PROPERTIES; CHARGE; MAGNETORESISTANCE; PEROVSKITES; ORDER;
D O I
10.1088/0022-3727/49/3/035001
中图分类号
O59 [应用物理学];
学科分类号
摘要
Magnetization measurements of La0.5Sr0.5Mn1-xAlxO3 (0 <= x <= 0.25) under pulsed high magnetic fields up to 50 T have been carried out, in which the Al3+ ions doping and magnetic field effects on the charge-ordering/antiferromagnetic to ferromagnetic phase transitions have been discussed. A triple-phase diagram with the critical field, doping level and temperature has been determined, in which the antiferromagntic and ferromagnetic phase boundaries were clearly defined. The change from long-range charge-ordered/antiferromagnetic phases to the robust short-range ones upon the Al3+-doping was observed. According to the experimental results, we assume that Al3+ ion doping at the Mn sites dilutes the Mn3+-O-Mn4+ network, weakens the double-exchange interaction and further suppresses the FM phase (metallic conduction), which leads to the critical magnetic fields destroying the antiferromagnetic order increase with the increase of the doping level.
引用
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页数:10
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