Inverted Quantum-Dot Light-Emitting Diodes Fabricated by All-Solution Processing

被引:86
作者
Zhang, Heng [1 ]
Li, Hanrun [1 ]
Sun, Xiaowei [1 ]
Chen, Shuming [1 ]
机构
[1] Southern Univ Sci & Technol, Dept Elect & Elect Engn, Shenzhen 518055, Peoples R China
基金
中国国家自然科学基金;
关键词
quantum dots; light-emitting diodes; inverted QD-LEDs; all-solution-processed; orthogonal solvents; intermixing; EFFICIENT; BRIGHT; DEVICES; PERFORMANCE;
D O I
10.1021/acsami.5b12737
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
All-solution processed, multilayer, and inverted quantum-dot light-emitting diodes (QD-LEDs) are developed in this work. To protect the QDs from dissolving by the solvents of upper layers, the solvents of poly(9-vinlycarbazole) (PVK) hole transporting layer are first investigated. The QD layer has been less affected by o-dichlorobenzene solvent than other typical solvents like, chloroform and chlorobenzene. Second, to deposit a hydrophilic poly(ethylenedioxythiophene)/polystyrenesulfonate (PEDOT:PSS) hole injection layer on top of hydrophobic PVK, the surface energy of the PEDOT:PSS is reduced by using isopropanol as the additive. With optimized conditions, the demonstrated QD-LEDs exhibit a maximum luminance of 16290 cd/m(2) and a peak current efficiency of 4.1 cd/A, which is the highest among the reported values. These results may offer a practicable platform for further research, leading to the achievement of all-solution processed, multilayer, and efficient inverted QD-LEDs.
引用
收藏
页码:5493 / 5498
页数:6
相关论文
共 28 条
  • [1] Colloidal quantum-dot light-emitting diodes with metal-oxide charge transport layers
    Caruge, J. M.
    Halpert, J. E.
    Wood, V.
    Bulovic, V.
    Bawendi, M. G.
    [J]. NATURE PHOTONICS, 2008, 2 (04) : 247 - 250
  • [2] All-Solution-Processed Inverted Quantum-Dot Light-Emitting Diodes
    Castan, Alice
    Kim, Hyo-Min
    Jang, Jin
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (04) : 2508 - 2515
  • [3] Real-time three-dimensional surface measurement by color encoded light projection
    Chen, S. Y.
    Li, Y. F.
    Guan, Q.
    Xiao, G.
    [J]. APPLIED PHYSICS LETTERS, 2006, 89 (11)
  • [4] Solution-processed, high-performance light-emitting diodes based on quantum dots
    Dai, Xingliang
    Zhang, Zhenxing
    Jin, Yizheng
    Niu, Yuan
    Cao, Hujia
    Liang, Xiaoyong
    Chen, Liwei
    Wang, Jianpu
    Peng, Xiaogang
    [J]. NATURE, 2014, 515 (7525) : 96 - 99
  • [5] CdSe/ZnS Quantum Dot Thin Film Formation by an Electrospray Deposition Process for Light-Emitting Devices
    Ho, My Duyen
    Kim, Namhun
    Kim, Daekyoung
    Cho, Sung Min
    Chae, Heeyeop
    [J]. SMALL, 2014, 10 (20) : 4142 - 4146
  • [6] Efficient Quantum Dot Light-Emitting Diodes by Controlling the Carrier Accumulation and Exciton Formation
    Ji, Wenyu
    Tian, Ye
    Zeng, Qinghui
    Qu, Songnan
    Zhang, Ligong
    Jing, Pengtao
    Wang, Jia
    Zhao, Jialong
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (16) : 14001 - 14007
  • [7] Contact Printing of Quantum Dot Light-Emitting Devices
    Kim, LeeAnn
    Anikeeva, Polina O.
    Coe-Sullivan, Seth A.
    Steckel, Jonathan S.
    Bawendi, Moungi G.
    Bulovic, Vladimir
    [J]. NANO LETTERS, 2008, 8 (12) : 4513 - 4517
  • [8] Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure
    Kwak, Jeonghun
    Bae, Wan Ki
    Lee, Donggu
    Park, Insun
    Lim, Jaehoon
    Park, Myeongjin
    Cho, Hyunduck
    Woo, Heeje
    Yoon, Do Y.
    Char, Kookheon
    Lee, Seonghoon
    Lee, Changhee
    [J]. NANO LETTERS, 2012, 12 (05) : 2362 - 2366
  • [9] Quantum Dot Light-Emitting Diode with Quantum Dots Inside the Hole Transporting Layers
    Leck, Kheng Swee
    Divayana, Yoga
    Zhao, Dewei
    Yang, Xuyong
    Abiyasa, Agus Putu
    Mutlugun, Evren
    Gao, Yuan
    Liu, Shuwei
    Tan, Swee Tiam
    Sun, Xiao Wei
    Demir, Hilmi Volkan
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (14) : 6535 - 6540
  • [10] Charge trapping in hybrid electroluminescence device containing CdSe/ZnS quantum dots embedded in a conducting poly(N-vinylcarbozole) layer
    Li, Fushan
    Guo, Tailiang
    Kim, Taewhan
    [J]. APPLIED PHYSICS LETTERS, 2010, 97 (06)