Edge-Oriented Tungsten Disulfide Catalyst Produced from Mesoporous WO3 for Highly Efficient Dye-Sensitized Solar Cells

被引:56
作者
Ahn, Sung Hoon
Manthiram, Arumugam [1 ]
机构
[1] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA
基金
新加坡国家研究基金会;
关键词
dye-sensitized solar cells; edge-oriented WS2; mesoporous WO3; rapid sulfurization; solar cells; COUNTER ELECTRODES; GRAPHENE NANOPLATELETS; HYDROGEN EVOLUTION; MOS2; NANOSHEETS; LOW-COST; FILMS; PERFORMANCE; LAYERS; SITES;
D O I
10.1002/aenm.201501814
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
An edge-oriented WS2 as a counter electrode (Cis reported for highly efficient dye-sensitized solar cells (DSSCs). Converted directly from a mesoporous interconnected WO3 structure by a rapid sulfurization process at high temperature, the oriented WS2 exposes a large number of active edge sites that lead to high catalytic activity toward triiodide reduction in DSSCs. The DSSC device with optimized edge-oriented WS2 CE exhibits a power conversion efficiency (PCE) of 8.85% at 100 mW cm-2, which is higher than that of Pt (7.20%). © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页数:7
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