Technical Note: Ensuring consistent, global measurements of very short-lived halocarbon gases in the ocean and atmosphere

被引:6
作者
Butler, J. H. [2 ]
Bell, T. G. [1 ]
Hall, B. D. [2 ]
Quack, B. [3 ]
Carpenter, L. J. [4 ]
Williams, J. [5 ]
机构
[1] Univ E Anglia, Sch Environm Sci, LGMAC, Norwich NR4 7TJ, Norfolk, England
[2] NOAA Earth Syst Res Lab, Global Monitoring Div, Boulder, CO USA
[3] Leibniz Inst Meereswissensch IFM GEOMAR, Kiel, Germany
[4] Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England
[5] Max Planck Inst Chem, D-55128 Mainz, Germany
基金
英国自然环境研究理事会;
关键词
MARINE BOUNDARY-LAYER; ATLANTIC-OCEAN; HALOGEN OXIDES; CHEMISTRY; TROPOSPHERE; AEROSOL; BROMINE; MODEL; AIR;
D O I
10.5194/acp-10-327-2010
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Very short-lived halocarbons are significant sources of reactive halogen in the marine boundary layer, and likely in the upper troposphere and lower stratosphere. Quantifying ambient concentrations in the surface ocean and atmosphere is essential for understanding the atmospheric impact of these trace gas fluxes. Despite the body of literature increasing substantially over recent years, calibration issues complicate the comparison of results and limit the utility of building larger-scale databases that would enable further development of the science (e.g. sea-air flux quantification, model validation, etc.). With this in mind, thirty-one scientists from both atmospheric and oceanic halocarbon communities in eight nations gathered in London in February 2008 to discuss the scientific issues and plan an international effort toward developing common calibration scales (< a href='http://tinyurl.com/c9cg58'target='_blank'> http://tinyurl.com/c9cg58 </a >). Here, we discuss the outputs from this meeting, suggest the compounds that should be targeted initially, identify opportunities for beginning calibration and comparison efforts, and make recommendations for ways to improve the comparability of previous and future measurements.
引用
收藏
页码:327 / 330
页数:4
相关论文
共 19 条
[1]  
[Anonymous], SCI ASSESSMENT OZONE
[2]   Using CHAMP radio occultation data to determine the top altitude of the Planetary Boundary Layer [J].
von Engeln, A ;
Teixeira, J ;
Wickert, J ;
Buehler, SA .
GEOPHYSICAL RESEARCH LETTERS, 2005, 32 (06) :1-4
[3]   Oceanic distributions and emissions of short-lived halocarbons [J].
Butler, James H. ;
King, Daniel B. ;
Lobert, Juergen M. ;
Montzka, Stephen A. ;
Yvon-Lewis, Shari A. ;
Hall, Bradley D. ;
Warwick, Nicola J. ;
Mondeel, Debra J. ;
Aydin, Murat ;
Elkins, James W. .
GLOBAL BIOGEOCHEMICAL CYCLES, 2007, 21 (01)
[4]   Air-sea fluxes of biogenic bromine from the tropical and North Atlantic Ocean [J].
Carpenter, L. J. ;
Jones, C. E. ;
Dunk, R. M. ;
Hornsby, K. E. ;
Woeltjen, J. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (05) :1805-1816
[5]  
Dorf M., 2005, Investigation of Inorganic Stratospheric Bromine using Balloon-Borne DOAS Measurements and Model Simulations
[6]  
KO MKW, 2003, SCI ASSESSMENT OZONE, pCH2
[7]   RADON MEASUREMENTS IN THE LOWER TROPICAL STRATOSPHERE - EVIDENCE FOR RAPID VERTICAL TRANSPORT AND DEHYDRATION OF TROPOSPHERIC AIR [J].
KRITZ, MA ;
ROSNER, SW ;
KELLY, KK ;
LOEWENSTEIN, M ;
CHAN, KR .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1993, 98 (D5) :8725-8736
[8]  
KURYLO MJ, 1999, SCI ASSESSMENT OZONE, pCH2
[9]   Evaluating ozone depletion from very short-lived halocarbons [J].
Olsen, SC ;
Hannegan, BJ ;
Zhu, X ;
Prather, MJ .
GEOPHYSICAL RESEARCH LETTERS, 2000, 27 (10) :1475-1478
[10]   Halogen cycling and aerosol pH in the Hawaiian marine boundary layer [J].
Pszenny, AAP ;
Moldanov , J ;
Keene, WC ;
Sander, R ;
Maben, JR ;
Martinez, M ;
Crutzen, PJ ;
Perner, D ;
Prinn, RG .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2004, 4 :147-168