Field-induced valence fluctuations in YbB12

被引:4
作者
Kurihara, R. [1 ]
Miyake, A. [1 ]
Tokunaga, M. [1 ]
Ikeda, A. [1 ]
Matsuda, Y. H. [1 ]
Miyata, A. [2 ,3 ]
Gorbunov, D., I [2 ,3 ]
Nomura, T. [1 ,2 ,3 ]
Zherlitsyn, S. [2 ,3 ]
Wosnitza, J. [2 ,3 ,4 ]
Iga, F. [5 ]
机构
[1] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan
[2] Helmholtz Zentrum Dresden Rossendorf, Hochfeld Magnetlab Dresden HLD EMFL, D-01328 Dresden, Germany
[3] Helmholtz Zentrum Dresden Rossendorf, Wurzburg Dresden Cluster Excellence Ct Qmat, D-01328 Dresden, Germany
[4] Tech Univ Dresden, Inst Festkorper & Mat Phys, D-01062 Dresden, Germany
[5] Ibaraki Univ, Inst Quantum Beam Sci, Mito, Ibaraki 3108512, Japan
关键词
X-RAY SPECTROSCOPY; ELASTIC PROPERTIES; ELECTRON; STATE;
D O I
10.1103/PhysRevB.103.115103
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We performed high-magnetic-field ultrasonic experiments on YbB12 up to 59 T to investigate the valence fluctuations in Yb ions. In zero field, the longitudinal elastic constant C-11, the transverse elastic constants C-44 and (C-11 - C-12)/2, and the bulk modulus C-B show a hardening with a change of curvature at around 35 K indicating a small contribution of valence fluctuations to the elastic constants. When high magnetic fields are applied at low temperatures, C-B exhibits a softening above a field-induced insulator-metal transition signaling field induced valence fluctuations. Furthermore, at elevated temperatures, the field-induced softening of C-B takes place at even lower fields and C-B decreases continuously with field. Our analysis using the multipole susceptibility based on a two-band model reveals that the softening of C-B originates from the enhancement of multipole-strain interaction in addition to the decrease of the insulator energy gap. This analysis indicates that field-induced valence fluctuations of Yb cause the instability of the bulk modulus C-B.
引用
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页数:14
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