Cathodes for Proton-Exchange-Membrane Fuel Cells Based on Ordered Mesoporous Carbon Supports

被引:11
|
作者
Lebedeva, Natalia P. [1 ]
Booij, Arend S. [1 ]
Janssen, Gaby J. M. [1 ]
机构
[1] Energy Res Ctr Netherlands ECN, NL-1755 ZG Petten, Netherlands
来源
关键词
D O I
10.1149/1.2982048
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Electrodes for the PEMFC were made from 40 wt% Pt on ordered mesoporous carbon (OMC) and their performance as cathodes in PEMFC fuel cells was evaluated. Good activity for the oxygen reduction reaction was found resulting in mass activities better than observed with commercial catalysts. The mesopores in the OMC were in the order of 3.6 nm, which did not prevent a high utilization of the Pt. However, the oxygen transport was very poor in these electrodes, suggesting the mesopores are easily blocked by ionomer and water.
引用
收藏
页码:2083 / 2092
页数:10
相关论文
共 50 条
  • [1] Sibunit Carbon-Based Cathodes for Proton-Exchange-Membrane Fuel Cells
    Lebedeva, N. P.
    Booij, A. S.
    Voropaev, I. N.
    Simonov, P. A.
    Romanenko, A. V.
    FUEL CELLS, 2009, 9 (04) : 439 - 452
  • [2] Performance of thin-film cathodes for proton-exchange-membrane fuel cells based on high-surface-area carbon supports
    Janssen, G. J. M.
    Sitters, E. F.
    JOURNAL OF POWER SOURCES, 2007, 171 (01) : 8 - 17
  • [3] Durability of Pt Catalysts Supported On Ordered Mesoporous Carbon for Proton Exchange Membrane Fuel Cells
    Kim, Nam-In
    Seong, Jinhae
    Yang, Min-Ji
    Cho, Sung-Hwa
    Park, Jun-Young
    Choi, Han-Shin
    Joo, Sang Hoon
    Kwon, Kyungjung
    POLYMER ELECTROLYTE FUEL CELLS 13 (PEFC 13), 2013, 58 (01): : 1277 - 1283
  • [4] Modeling of the Mass Transfer in Proton-Exchange-Membrane Fuel Cells
    S. A. Grigor'ev
    Yu. R. Alanakyan
    V. N. Fateev
    V. D. Rusanov
    Doklady Physical Chemistry, 2002, 382 : 31 - 34
  • [5] A gas distributor design for proton-exchange-membrane fuel cells
    Nguyen, TV
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1996, 143 (05) : L103 - L105
  • [6] Modeling of the mass transfer in proton-exchange-membrane fuel cells
    Grigor'ev, SA
    Alanakyan, YR
    Fateev, VN
    Rusanov, AVD
    DOKLADY PHYSICAL CHEMISTRY, 2002, 382 (4-6) : 31 - 34
  • [7] Graphene and carbon nanotube structures supported on mesoporous xerogel carbon as catalysts for oxygen reduction reaction in proton-exchange-membrane fuel cells
    Arbizzani, Catia
    Righi, Sara
    Soavi, Francesca
    Mastragostino, Marina
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2011, 36 (08) : 5038 - 5046
  • [8] Application and optimization of carbon supports in proton exchange membrane fuel cells
    Feng B.
    Lu M.
    Huang Z.
    Chang Y.
    Cui Z.
    Huagong Xuebao/CIESC Journal, 2024, 75 (04): : 1469 - 1484
  • [9] Comparing different production technologies for proton-exchange-membrane fuel cells
    Fischer, A
    Veziridis, Z
    Wendt, H
    HYDROGEN ENERGY PROGRESS XI, VOLS 1-3, 1996, : 2523 - 2530
  • [10] Durability of Sulfonated Aromatic Polymers for Proton-Exchange-Membrane Fuel Cells
    Hou, Hongying
    Di Vona, Maria Luisa
    Knauth, Philippe
    CHEMSUSCHEM, 2011, 4 (11) : 1526 - 1536