Changes in heavy metal mobility and availability from contaminated wetland soil remediated with combined biochar-compost

被引：311
作者：
Liang, Jie [1 ,2 ]
Yang, Zhaoxue [1 ,2 ]
Tang, Lin [1 ,2 ]
Zeng, Guangming [1 ,2 ]
Yu, Man [3 ]
Li, Xiaodong [1 ,2 ]
Wu, Haipeng [4 ]
Qian, Yingying [1 ,2 ]
Li, Xuemei [1 ,2 ]
Luo, Yuan [1 ,2 ]
机构：
[1] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China
[2] Hunan Univ, Minist Educ, Key Lab Environm Biol & Pollut Control, Changsha 410082, Hunan, Peoples R China
[3] Zhejiang Acad Agr Sci, Environm Resources & Soil Fertilizer Inst, Hangzhou 310021, Zhejiang, Peoples R China
[4] Changjiang River Sci Res Inst, Wuhan 430010, Peoples R China
来源：
CHEMOSPHERE | 2017年 / 181卷
基金：
中国国家自然科学基金;
关键词：
Wetland soil; Heavy metals; Combined biochar-compost; Soil physicochemical properties; Availability; Speciation distribution; DONGTING LAKE WETLAND; BACTERIAL COMMUNITY STRUCTURE; ORDERED MESOPOROUS CARBON; DISSOLVED ORGANIC-MATTER; RISK-ASSESSMENT; SEWAGE-SLUDGE; MIDDLE CHINA; PADDY SOIL; ADSORPTION CHARACTERISTICS; COMBINED AMENDMENTS;
D O I：
10.1016/j.chemosphere.2017.04.081
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
The combination of biochar and compost has been proven to be effective in heavy metals contaminated wetland soil restoration. However, the influence of different proportions between biochar and compost on immobilization of heavy metals in soil has been less studied up to date. Therefore, we investigated the effect of different ratios of biochar-compost mixtures on availability and speciation distribution of heavy metals (Cd, Zn and Cu) in wetland soil. The results showed that applying all amendment combinations into wetland soil increased gradually the total organic carbon (TOC) and water-extract organic carbon (WEOC) as the compost percentage rose in biochar-composts. The higher pH was obtained in a certain biochar addition (20% and 40%) in combinations due to efficient interaction of biochar with compost. All amendments could significantly decrease availability of Cd and Zn mainly from pH change, but increase available Cu concentration as the result of increased water-extract organic carbon and high total Cu content in compost. Moreover, amendments can decrease easily exchangeable fraction and increase reducible of Cd and Zn greatly with increase of compost content in combinations, while amendments containing compost promote transformation of Cu from Fe/Mn oxide and residual fractions to organic bindings. These results demonstrate that different ratios of biochar and compost have a significant effect on availability and speciation of heavy metals in multi-metal-contaminated wetland soil. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码：281 / 288
页数：8
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