Kinetics of catalytically activated duplication in aggregation growth

被引:2
作者
Wang Hai-Feng [1 ,2 ]
Lin Zhen-Quan [3 ]
Gao Yan [1 ,2 ]
Xu Chao [1 ,2 ]
机构
[1] Shihezi Univ, Key Lab Ecophys, Shihezi 832003, Peoples R China
[2] Shihezi Univ, Dept Phys, Teachers Coll, Shihezi 832003, Peoples R China
[3] Wenzhou Univ, Dept Phys, Wenzhou 325027, Peoples R China
基金
芬兰科学院; 中国国家自然科学基金;
关键词
aggregation; catalytically activated reaction; rate equation; kinetic behavior; ANNIHILATION PROCESSES; CHAIN; COAGULATION; GELATION; DNA; UNIVERSALITY; REPLICATION; CONSTANT; BEHAVIOR; EQUATION;
D O I
10.1088/1674-1056/18/8/074
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We propose a catalytically activated duplication model to mimic the coagulation and duplication of the DNA polymer system under the catalysis of the primer RNA. In the model, two aggregates of the same species can coagulate themselves and a DNA aggregate of any size can yield a new monomer or double itself with the help of RNA aggregates. By employing the mean-field rate equation approach we analytically investigate the evolution behaviour of the system. For the system with catalysis-driven monomer duplications, the aggregate size distribution of DNA polymers a(k)(t) always follows a power law in size in the long-time limit, and it decreases with time or approaches a time-independent steady-state form in the case of the duplication rate independent of the size of the mother aggregates, while it increases with time increasing in the case of the duplication rate proportional to the size of the mother aggregates. For the system with complete catalysis-driven duplications, the aggregate size distribution a(k)(t) approaches a generalized or modified scaling form.
引用
收藏
页码:3577 / 3584
页数:8
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