The microscopic structure of charge density waves in underdoped YBa2Cu3O6.54 revealed by X-ray diffraction

被引:80
作者
Forgan, E. M. [1 ]
Blackburn, E. [1 ]
Holmes, A. T. [1 ]
Briffa, A. K. R. [1 ]
Chang, J. [2 ]
Bouchenoire, L. [3 ,4 ]
Brown, S. D. [3 ,4 ]
Liang, Ruixing [5 ]
Bonn, D. [5 ]
Hardy, W. N. [5 ]
Christensen, N. B. [6 ]
von Zimmermann, M. [7 ]
Huecker, M. [8 ]
Hayden, S. M. [9 ]
机构
[1] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England
[2] Univ Zurich, Inst Phys, CH-8057 Zurich, Switzerland
[3] European Synchrotron Radiat Facil, XMaS, F-38043 Grenoble, France
[4] Univ Liverpool, Dept Phys, Liverpool L69 3BX, Merseyside, England
[5] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada
[6] Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark
[7] Deutsches Elektronen Synchrotron DESY, D-22603 Hamburg, Germany
[8] Brookhaven Natl Lab, Condensed Matter Phys Mat Sci Dept, Upton, NY 11973 USA
[9] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England
来源
NATURE COMMUNICATIONS | 2015年 / 6卷
基金
英国工程与自然科学研究理事会; 瑞士国家科学基金会; 加拿大自然科学与工程研究理事会;
关键词
ORDER; SUPERCONDUCTIVITY;
D O I
10.1038/ncomms10064
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Charge density wave (CDW) order appears throughout the underdoped high-temperature cuprate superconductors, but the underlying symmetry breaking and the origin of the CDW remain unclear. We use X-ray diffraction to determine the microscopic structure of the CDWs in an archetypical cuprate YBa2Cu3O6.54 at its superconducting transition temperature similar to 60 K. We find that the CDWs in this material break the mirror symmetry of the CuO2 bilayers. The ionic displacements in the CDWs have two components, which are perpendicular and parallel to the CuO2 planes, and are out of phase with each other. The planar oxygen atoms have the largest displacements, perpendicular to the CuO2 planes. Our results allow many electronic properties of the underdoped cuprates to be understood. For instance, the CDWs will lead to local variations in the electronic structure, giving an explicit explanation of density-wave states with broken symmetry observed in scanning tunnelling microscopy and soft X-ray measurements.
引用
收藏
页数:7
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