Determining the nonequilibrium criticality of a Gardner transition via a hybrid study of molecular simulations and machine learning

被引:26
作者
Li, Huaping [1 ,2 ,3 ]
Jin, Yuliang [4 ,5 ]
Jiang, Ying [1 ,2 ]
Chen, Jeff Z. Y. [6 ]
机构
[1] Beihang Univ, Sch Chem, Beijing 100191, Peoples R China
[2] Beihang Univ, Ctr Soft Matter Phys & Its Applicat, Beijing 100191, Peoples R China
[3] Univ Chinese Acad Sci, Wenzhou Inst, Wenzhou 325000, Peoples R China
[4] Chinese Acad Sci, Inst Theoret Phys, Beijing 100190, Peoples R China
[5] Univ Chinese Acad Sci, Sch Phys Sci, Beijing 100049, Peoples R China
[6] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada
基金
中国国家自然科学基金; 加拿大自然科学与工程研究理事会; 中国博士后科学基金;
关键词
glass; Gardner transition; machine learning; critical exponents; SPIN-GLASS;
D O I
10.1073/pnas.2017392118
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Apparent critical phenomena, typically indicated by growing correlation lengths and dynamical slowing down, are ubiquitous in nonequilibrium systems such as supercooled liquids, amorphous solids, active matter, and spin glasses. It is often challenging to determine if such observations are related to a true second-order phase transition as in the equilibrium case or simply a crossover and even more so to measure the associated critical exponents. Here we show that the simulation results of a hard-sphere glass in three dimensions are consistent with the recent theoretical prediction of a Gardner transition, a continuous nonequilibrium phase transition. Using a hybrid molecular simulation-machine learning approach, we obtain scaling laws for both finite-size and aging effects and determine the critical exponents that traditional methods fail to estimate. Our study provides an approach that is useful to understand the nature of glass transitions and can be generalized to analyze other nonequilibrium phase transitions.
引用
收藏
页数:7
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