Nitrogen self-doped porous carbon material derived from metal-organic framework for high-performance super-capacitors

被引：32

作者：

Zhang Dongqiang ^{[1
]}

Wang Jiaxi ^{[2
]}

Wang Qian ^{[1
]}

Huang Siyun ^{[1
]}

Feng Huixia ^{[1
]}

Luo Heming ^{[1
]}

机构：

[1] Lan Zhou Univ Technol, Sch Petrochem Engn, Lanzhou, Gansu, Peoples R China

[2] Nankai Univ, Sch Mat Sci & Engn Chem, Tianjin, Peoples R China

来源：

JOURNAL OF ENERGY STORAGE | 2019年 / 25卷

关键词：

Metal-organic frameworks; Nitrogen self-doped porous carbon; Electrochemical; Specific capacitance; Super-capacitors; ZEOLITIC IMIDAZOLATE FRAMEWORK; NANOPOROUS CARBONS; DIRECT CARBONIZATION; FACILE SYNTHESIS; SUPERCAPACITORS; ADSORPTION; STABILITY; RETENTION; WASTE;

D O I：

10.1016/j.est.2019.100904

中图分类号：

TE [石油、天然气工业]; TK [能源与动力工程];

学科分类号：

0807 ; 0820 ;

摘要：

Metal-organic framework materials (MOFs) have extensive application prospects as carbon precursors for super-capacitors are of great interest due to diverse microstructures, uniform pore size, high porosity, and tunable pore parameters. Here, nitrogen self-doped porous carbon materials (ZABC-T) derived from [Zn-2(BTEC)(0.5)(ATZ)(2)(H2O)(3)]center dot H2O (ZAB) have been prepared via a facile and fast carbonization method at different temperature. The nitrogen self-doped porous carbon material (ZABC-800) features a high specific surface area of 1008 m(2) g(-1) and high nitrogen content of 4.09%. Consequently, the ZABC-800 shows an excellent specific capacitance of 316.3 F g(-1) at 1.0 A g(-1), superior rate capacity, and remarkable cycling stability (81.9% retention after 5000 cycles). This work indicates that the ZABC-T has a great potential as electrode materials for high performance super-capacitors.

引用

页数：8

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