Recent Advances in Metal-Organic Frameworks for Photo-/Electrocatalytic CO2 Reduction

被引：57

作者：

Wang, Qingqing ^{[1
,2
,3
,4
]}

Zhang, Yao ^{[1
,2
,3
,4
]}

Lin, Huijuan ^{[2
,3
,4
]}

Zhu, Jixin ^{[1
,2
,3
,4
]}

机构：

[1] NPU, SIFE, 127 West Youyi Rd, Xian 710072, Shaanxi, Peoples R China

[2] Nanjing Tech Univ NanjingTech, KLOFE, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China

[3] Nanjing Tech Univ NanjingTech, IAM, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China

[4] Nanjing Tech Univ NanjingTech, Jiangsu Natl Synerget Innovat Ctr Adv Mat SICAM, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China

来源：

CHEMISTRY-A EUROPEAN JOURNAL | 2019年 / 25卷 / 62期

基金：

中国国家自然科学基金;

关键词：

CO2; reduction; electrocatalysis; metal-organic frameworks; molecular tuning; photocatalysis; CARBON-DIOXIDE; PHOTOCATALYTIC REDUCTION; ELECTROCHEMICAL REDUCTION; ELECTROCATALYTIC REDUCTION; TUNABLE PLATFORM; WATER OXIDATION; ENERGY-STORAGE; EFFICIENT; CATALYSTS; DRIVEN;

D O I：

10.1002/chem.201902203

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Considerable attention has been paid to the utilization of CO2, an abundant carbon source in nature. In this regard, porous catalysts have been eagerly explored with excellent performance for photo-/electrocatalytic reduction of CO2 to high valued products. Metal-organic frameworks (MOFs), featuring large surface area, high porosity, tunable composition and unique structural characteristics, have been widely exploited in catalytic CO2 reduction. This Minireview first reports the current progress of MOFs in CO2 reduction. Then, a specific interest is focused on MOFs in photo-/electrocatalytic reduction of CO2 by modifying their metal centers, organic linkers, and pores. Finally, the future directions of study are also highlighted to satisfy the requirement of practical applications.

引用

页码：14026 / 14035

页数：10

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