Trimetallic TriStar Nanostructures: Tuning Electronic and Surface Structures for Enhanced Electrocatalytic Hydrogen Evolution

被引:186
作者
Du, Nana [1 ,2 ,3 ]
Wang, Chengming [1 ,2 ]
Wang, Xijun [1 ,2 ]
Lin, Yue [1 ,2 ]
Jiang, Jun [1 ,2 ]
Xiong, Yujie [1 ,2 ]
机构
[1] Chinese Acad Sci, Hefei Sci Ctr, iChEM Collaborat Innovat Ctr Chem Energy Mat, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
[2] Univ Sci & Technol China, Sch Chem & Mat Sci, Hefei 230026, Anhui, Peoples R China
[3] Fuyang Normal Coll, Coll Chem & Chem Engn, Fuyang 236041, Anhui, Peoples R China
关键词
CATALYTIC-ACTIVITY; REDUCTION; PLATINUM; METAL; NANOPARTICLES; TRANSITION; CU; GOLD; ELECTROCHEMISTRY; PERFORMANCE;
D O I
10.1002/adma.201504785
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
PtFeCo alloy nanostructures in a TriStar shape with tunable Fe and Co content are developed for the electrocatalytic hydrogen evolution reaction (HER). With electronic and surface structures well-tailored, the PtFeCo nanostructures exhibit dramatically enhanced performance in HER against commercial Pt/C and other Pt-based nanoparticles.
引用
收藏
页码:2077 / +
页数:9
相关论文
共 43 条
  • [1] [Anonymous], ANGEW CHEM INT ED
  • [2] Surface Polarization Matters: Enhancing the Hydrogen-Evolution Reaction by Shrinking Pt Shells in Pt-Pd-Graphene Stack Structures
    Bai, Song
    Wang, Chengming
    Deng, Mingsen
    Gong, Ming
    Bai, Yu
    Jiang, Jun
    Xiong, Yujie
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2014, 53 (45) : 12120 - 12124
  • [3] Highly catalytic active PtNiCu nanochains for hydrogen evolution reaction
    Cao, Xia
    Han, Yu
    Gao, Caizhen
    Xu, Ying
    Huang, Xiaomin
    Willander, Magnus
    Wang, Ning
    [J]. NANO ENERGY, 2014, 9 : 301 - 308
  • [4] Highly Crystalline Multimetallic Nanoframes with Three-Dimensional Electrocatalytic Surfaces
    Chen, Chen
    Kang, Yijin
    Huo, Ziyang
    Zhu, Zhongwei
    Huang, Wenyu
    Xin, Huolin L.
    Snyder, Joshua D.
    Li, Dongguo
    Herron, Jeffrey A.
    Mavrikakis, Manos
    Chi, Miaofang
    More, Karren L.
    Li, Yadong
    Markovic, Nenad M.
    Somorjai, Gabor A.
    Yang, Peidong
    Stamenkovic, Vojislav R.
    [J]. SCIENCE, 2014, 343 (6177) : 1339 - 1343
  • [5] Supportless Pt and PtPd nanotubes as electrocatalysts for oxygen-reduction reactions
    Chen, Zhongwei
    Waje, Mahesh
    Li, Wenzhen
    Yan, Yushan
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2007, 46 (22) : 4060 - 4063
  • [6] Greeley J, 2009, NAT CHEM, V1, P552, DOI [10.1038/nchem.367, 10.1038/NCHEM.367]
  • [7] Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
    Greeley, Jeff
    Jaramillo, Thomas F.
    Bonde, Jacob
    Chorkendorff, I. B.
    Norskov, Jens K.
    [J]. NATURE MATERIALS, 2006, 5 (11) : 909 - 913
  • [8] FePt and CoPt Nanowires as Efficient Catalysts for the Oxygen Reduction Reaction
    Guo, Shaojun
    Li, Dongguo
    Zhu, Huiyuan
    Zhang, Sen
    Markovic, Nenad M.
    Stamenkovic, Vojislav R.
    Sun, Shouheng
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (12) : 3465 - 3468
  • [9] FePt Nanoparticles Assembled on Graphene as Enhanced Catalyst for Oxygen Reduction Reaction
    Guo, Shaojun
    Sun, Shouheng
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (05) : 2492 - 2495
  • [10] WHY GOLD IS THE NOBLEST OF ALL THE METALS
    HAMMER, B
    NORSKOV, JK
    [J]. NATURE, 1995, 376 (6537) : 238 - 240