A simple but effective design to enhance the performance and durability of direct carbon solid oxide fuel cells

被引:12
作者
Kong, Wei [1 ]
Han, Zhen [1 ]
Lu, Siyu [1 ]
Ni, Meng [2 ]
机构
[1] Jiangsu Univ Sci & Technol, Sch Energy & Power, Zhenjiang 212003, Jiangsu, Peoples R China
[2] Hong Kong Polytech Univ, Dept Bldg & Real Estate, Bldg Energy Res Grp, Hung Hom,Kowloon, Hong Kong, Peoples R China
基金
美国国家科学基金会;
关键词
Direct carbon fuel cell; Solid oxide fuel cell; Boudouard reaction; Temperature; Carbon;
D O I
10.1016/j.apenergy.2021.116586
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The development of high-performance and durable direct carbon solid oxide fuel cells requires that the rate of the Boudouard reaction is enhanced without significantly increasing the fuel cell temperature. Herein, a simple design is proposed to improve the performance of direct carbon solid oxide fuel cells by introducing a heat bar into the anode carbon compartment. This design is evaluated numerically using a 2D model. After model validation, parametric simulations are conducted to compare the performance of direct carbon solid oxide fuel cells with and without the heat bar. The heat bar improves the temperature uniformity of the fuel cell and enhances the local temperature in the carbon compartment. As a result, the Boudouard reaction rate is enhanced by 14% at a voltage of 0.6 V, leading to a performance enhancement of 4.1%. The heat bar significantly reduces the difference between the maximum and minimum temperatures in the fuel cell by 40%, leading to improved durability. This design becomes more effective when using a heat bar with a high thermal conductivity and at lower operating voltages. This study clearly demonstrates that this new design is a simple but effective method for enhancing the performance and durability of direct carbon solid oxide fuel cells.
引用
收藏
页数:8
相关论文
共 25 条
  • [1] Cai W, 2018, INT J ENERGY RES
  • [2] A high performance direct carbon solid oxide fuel cell fueled by Ca-loaded activated carbon
    Cai, Weizi
    Liu, Jiang
    Yu, Fangyong
    Zhou, Qian
    Zhang, Yapeng
    Wang, Xiaoqiang
    Liu, Meilin
    Ni, Meng
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (33) : 21167 - 21176
  • [3] An investigation on the kinetics of direct carbon solid oxide fuel cells
    Cai, Weizi
    Liu, Jiang
    Xie, Yongmin
    Xiao, Jie
    Liu, Meilin
    [J]. JOURNAL OF SOLID STATE ELECTROCHEMISTRY, 2016, 20 (08) : 2207 - 2216
  • [4] ELECTRICAL-PROPERTIES OF CERIA-BASED OXIDES AND THEIR APPLICATION TO SOLID OXIDE FUEL-CELLS
    EGUCHI, K
    SETOGUCHI, T
    INOUE, T
    ARAI, H
    [J]. SOLID STATE IONICS, 1992, 52 (1-3) : 165 - 172
  • [5] A steel slag-derived Boudouard reaction catalyst for improved performance of direct carbon solid oxide fuel cells
    Jiao, Yong
    Wang, Chongyang
    Zhang, Liqin
    An, Wenting
    Zhou, Na
    Yang, Guangming
    Wang, Wei
    Zhou, Wei
    Li, Si-Dian
    [J]. INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2019, 43 (13) : 6970 - 6982
  • [6] A novel interconnector design of SOFC
    Kong, Wei
    Han, Zhen
    Lu, Siyu
    Gao, Xiang
    Wang, Xiaorong
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2020, 45 (39) : 20329 - 20338
  • [7] Optimization of the Interconnect Ribs for a Cathode-Supported Solid Oxide Fuel Cell
    Kong, Wei
    Gao, Xiang
    Liu, Shixue
    Su, Shichuan
    Chen, Daifen
    [J]. ENERGIES, 2014, 7 (01): : 295 - 313
  • [8] Electrochemical Oxidation of Carbon at High Temperature: Principles and Applications
    Liu, Jiang
    Zhou, Mingyang
    Zhang, Yapeng
    Liu, Peipei
    Liu, Zhijun
    Xie, Yongmin
    Cai, Weizi
    Yu, Fangyong
    Zhou, Qian
    Wang, Xiaoqiang
    Ni, Meng
    Liu, Meilin
    [J]. ENERGY & FUELS, 2018, 32 (04) : 4107 - 4117
  • [9] A novel direct carbon fuel cell by approach of tubular solid oxide fuel cells
    Liu, Renzhu
    Zhao, Chunhua
    Li, Junliang
    Zeng, Fanrong
    Wang, Shaorong
    Wen, Tinglian
    Wen, Zhaoyin
    [J]. JOURNAL OF POWER SOURCES, 2010, 195 (02) : 480 - 482
  • [10] Lu S, 2019, INT J HYDROGEN ENERG