Riverine dissolved organic carbon and its optical properties in a permafrost region of the Upper Heihe River basin in the Northern Tibetan Plateau

被引:33
作者
Gao, Tanguang [1 ]
Kang, Shichang [2 ,3 ]
Chen, Rensheng [2 ]
Zhang, Taigang [1 ]
Zhang, Tingjun [1 ]
Han, Chuntan [2 ]
Tripathee, Lekhendra [2 ]
Sillanpaa, Mika [4 ]
Zhang, Yulan [2 ,3 ]
机构
[1] Lanzhou Univ, Key Lab Western Chinas Environm Syst, Minist Educ, Coll Earth & Environm Sci, Lanzhou 730000, Gansu, Peoples R China
[2] Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Gansu, Peoples R China
[3] CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China
[4] Lappeenranta Univ Technol, Lab Green Chem, Mikkeli 50130, Finland
基金
中国国家自然科学基金;
关键词
DOC; River water; Permafrost; Absorbance; Spectral slope; Tibetan Plateau; MATTER COMPOSITION; MOLECULAR-WEIGHT; CLIMATE-CHANGE; ABSORPTION; EXPORT; CRYOSPHERE; MOUNTAINS; GLACIER; RUNOFF; COVER;
D O I
10.1016/j.scitotenv.2019.05.478
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Riverine dissolved organic carbon (DOC) and its optical properties were investigated in two sub-river basins (Yeniugou and Hulugou river) of the Upper Heihe river basin in the northern Tibetan Plateau. The results showed that DOC concentrations ranged from 025 to 12.2 and 0.18-1.04 mg L-1 for Yeniugou and Hulugou river basin with an average of 0.82 and 0.33 mg L-1, respectively. Export of DOC from the studied river (YNG: similar to 0.86 Gg C yr(-1)) was lesser compared with other large river in the Tibetan Plateau and Arctic regions because of the small drainage area and lower DOC concentrations. There exhibited significant seasonality for DOC in Yeniugou river basin with higher values observed during late spring and summer; however, no such distinct trend was observed for DOC in the studied rivers of Hulugou river basin. In contrast, total dissolved nitrogen showed a slightly lower value during the summer season. A strong relationship was determined between DOC concentrations and spectral UV absorbance at 254 nm (SUVA(254)), absorption coefficients and spectral slope for both sub-river basins, attributing that the riverine DOM in the northern Tibetan Plateau has a remarkably high content of aromatic compounds in late spring and summer. Considering the less snow cover percentage, this study highlights the potential impacts of permafrost thaw on the riverine DOC and its characteristics in the permafrost region under climate change. (C) 2019 Elsevier B.V. All rights reserved.
引用
收藏
页码:370 / 381
页数:12
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