Occurrence of polybrominated diphenyl ethers (PBDEs) in foodstuffs in Italy and implications for human exposure

被引:68
|
作者
Martellini, Tania [1 ]
Diletti, Gianfranco [2 ]
Scortichini, Giampiero [3 ]
Lolini, Meri [4 ]
Lanciotti, Eudes [5 ]
Katsoyiannis, Athanasios [6 ]
Cincinelli, Alessandra [1 ]
机构
[1] Univ Florence, Dept Chem Ugo Schiff, Via Lastruccia 3, I-50019 Florence, Italy
[2] Ist Zooprofilatt Sperimentale Abruzzo Molise G Ca, Natl Reference Lab Dioxins & PCBs Food & Feed, Via Campo Boario, I-64100 Teramo, Italy
[3] Ist Zooprofilatt Sperimentale Umbria & Marche, Dept Food & Feed Chem, Via G Salvemini, I-06126 Perugia, Italy
[4] Reg Agcy Environm Protect Reg Tuscany ARPAT, Via Ponte Mosse, I-50100 Florence, Italy
[5] Univ Florence, Dept Publ Hlth, Viale Morgagni 48, I-50134 Florence, Italy
[6] Norwegian Inst Air Res NILU, FRAM, High North Res Ctr Climate & Environm, NO-9296 Tromso, Norway
关键词
PBDEs; Foodstuffs; GC-NCI-MS; Human exposure; BROMINATED FLAME RETARDANTS; IN-HOUSE DUST; HEALTH-RISKS; DIETARY EXPOSURE; POLYCHLORINATED-BIPHENYLS; CHLORINATED PESTICIDES; FOOD-CONSUMPTION; TEMPORAL TRENDS; MARKET BASKET; BODY BURDENS;
D O I
10.1016/j.fct.2015.12.026
中图分类号
TS2 [食品工业];
学科分类号
0832 ;
摘要
Polybrominated diphenyl ethers (PBDEs) were determined in various foodstuffs in Italy and the dietary intake was estimated. PBDEs were detected in all analysed samples at concentrations that spanned over five orders of magnitude. The most abundant congeners were the BDE-209, followed by BDE-47 and BDE-99. Fish oil and milk samples showed the highest PBDE concentrations among all samples. The daily dietary intake values were found to be in good agreement or higher to literature values, impacted mainly from the contribution of the analysed dairy products. The cancer risk values estimated for BDE-209 indicated that this specific risk associated with the studied foodstuffs is limited. Italy is one of the world-leading countries in the production of furniture and clothes and has extremely developed medium enterprise industrial sector, where PBDEs were historically used suggesting that their occurrence may be linked to these activities. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:32 / 38
页数:7
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