Hard and soft landing of mass selected Ag clusters on Pt(111)

被引:46
作者
Bromann, K
Brune, H
Felix, C
Harbich, W
Monot, R
Buttet, J
Kern, K
机构
[1] Inst. de Phys. Expérimentale, EPFL
关键词
clusters; epitaxy; low index single crystal surfaces; platinum; scanning tunneling microscopy; silver; surface structure; morphology; roughness; and topography;
D O I
10.1016/S0039-6028(96)01544-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Mass selected Ag-n clusters (n = 1, 7, 19) from a secondary ion source have been deposited onto a Pt(111) substrate at low temperature. The surface and resulting cluster morphology have subsequently been characterized within the same UHV chamber by variable temperature STM as a function of cluster size, kinetic impact energy, and substrate temperature. The kinetic energy per cluster atom was found to be the decisive parameter for a controlled deposition. Noble gas buffer layers (approximate to 10 ML Ar), which were pre-adsorbed onto the surface at low temperatures, were found to efficiently dissipate the impact energy opening up the possibility of soft landing clusters with elevated kinetic energy.
引用
收藏
页码:1051 / 1055
页数:5
相关论文
共 16 条
[1]   EXPERIMENTAL-OBSERVATION OF FAST DIFFUSION OF LARGE ANTIMONY CLUSTERS ON GRAPHITE SURFACES [J].
BARDOTTI, L ;
JENSEN, P ;
HOAREAU, A ;
TREILLEUX, M ;
CABAUD, B .
PHYSICAL REVIEW LETTERS, 1995, 74 (23) :4694-4697
[2]   SCALING ANALYSIS OF DIFFUSION-MEDIATED ISLAND GROWTH IN SURFACE-ADSORPTION PROCESSES [J].
BARTELT, MC ;
EVANS, JW .
PHYSICAL REVIEW B, 1992, 46 (19) :12675-12687
[3]   KINETIC PROCESSES IN METAL EPITAXY STUDIED WITH VARIABLE-TEMPERATURE STM - AG/PT(111) [J].
BRUNE, H ;
RODER, H ;
BROMANN, K ;
KERN, K .
THIN SOLID FILMS, 1995, 264 (02) :230-235
[4]   MECHANISM OF THE TRANSITION FROM FRACTAL TO DENDRITIC GROWTH OF SURFACE AGGREGATES [J].
BRUNE, H ;
ROMAINCZYK, C ;
RODER, H ;
KERN, K .
NATURE, 1994, 369 (6480) :469-471
[5]   MICROSCOPIC VIEW OF NUCLEATION ON SURFACES [J].
BRUNE, H ;
RODER, H ;
BORAGNO, C ;
KERN, K .
PHYSICAL REVIEW LETTERS, 1994, 73 (14) :1955-1958
[6]   CONTROLLED DEPOSITION AND GLASSIFICATION OF COPPER NANOCLUSTERS [J].
CHENG, HP ;
LANDMAN, U .
JOURNAL OF PHYSICAL CHEMISTRY, 1994, 98 (13) :3527-3537
[7]   PHOTOEMISSION FROM MASS-SELECTED MONODISPERSED PT CLUSTERS [J].
EBERHARDT, W ;
FAYET, P ;
COX, DM ;
FU, Z ;
KALDOR, A ;
SHERWOOD, R ;
SONDERICKER, D .
PHYSICAL REVIEW LETTERS, 1990, 64 (07) :780-784
[8]   Deposition and growth of noble metal clusters on graphite [J].
Francis, GM ;
Goldby, IM ;
Kuipers, L ;
vonIssendorff, B ;
Palmer, RE .
JOURNAL OF THE CHEMICAL SOCIETY-DALTON TRANSACTIONS, 1996, (05) :665-671
[9]   THIN-FILMS FROM ENERGETIC CLUSTER-IMPACT - EXPERIMENT AND MOLECULAR-DYNAMICS SIMULATIONS [J].
HABERLAND, H ;
INSEPOV, Z ;
KARRAIS, M ;
MALL, M ;
MOSELER, M ;
THURNER, Y .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1993, 80-1 :1320-1323
[10]  
JOHN PMS, 1992, PHYS REV LETT, V69, P1467