Synthesis of three dimensional extended conjugated polyimide and application as sodium-ion battery anode

被引：92

作者：

Li, Zhongtao ^{[1
]}

Zhou, Jingyan ^{[1
]}

Xu, Rongfei ^{[1
]}

Liu, Shuiping ^{[2
]}

Wang, Yuankun ^{[1
]}

Li, Peng ^{[1
]}

Wu, Wenting ^{[1
]}

Wu, Mingbo ^{[1
]}

机构：

[1] China Univ Petr, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China

[2] Donghua Univ, State Key Lab Modificat Chem Fibers & Polymer Mat, Shanghai 201620, Peoples R China

来源：

CHEMICAL ENGINEERING JOURNAL | 2016年 / 287卷

基金：

中国国家自然科学基金;

关键词：

Polyimide; Sodium-ion battery; Anode; Electrochemical performance; ORGANIC ELECTRODE MATERIALS; GRAPHENE OXIDE; CARBON; PERFORMANCE; STORAGE; CHARGE;

D O I：

10.1016/j.cej.2015.11.063

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

Two covalent polyimides with different conjugated subunits have been synthesized as sodium-ion batteries anode. The melamine and two commercially available dianhydrides have been adopted as building blocks to fabricate 3D extended covalent frameworks, which are consisted of electron withdrawing amide groups and triazine rings to coordination with Na ions. The results revealed that cross-linked polymer exhibits excellent durability and rate capacity (88.8 mAh g(-1) at a current density of 5.0 A g(-1) after 1000 cycles), which provides a promising candidate for high performance Na-ion battery anode. (C) 2015 Elsevier B.V. All rights reserved.

引用

页码：516 / 522

页数：7

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