Metallic few-layered VSe2 nanosheets: high two-dimensional conductivity for flexible in-plane solid-state supercapacitors

被引:106
作者
Wang, Chaolun [1 ]
Wu, Xing [1 ]
Ma, Yonghui [2 ]
Mu, Gang [2 ]
Li, Yaoyi [3 ]
Luo, Chen [1 ]
Xu, Hejun [1 ]
Zhang, Yuanyuan [1 ]
Yang, Jing [1 ]
Tang, Xiaodong [1 ]
Zhang, Jian [1 ,6 ]
Bao, Wenzhong [4 ]
Duan, Chungang [1 ,5 ]
机构
[1] East China Normal Univ, Dept Elect Engn, Shanghai Key Lab Multidimens Informat Proc, Key Lab Polar Mat & Devices MOE, 500 Dongchuan Rd, Shanghai 200241, Peoples R China
[2] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China
[3] Shanghai Jiao Tong Univ, Sch Phys & Astron, Key Lab Arti cial Struct & Quantum Control MOE, 800 Dongchuan Rd, Shanghai 200240, Peoples R China
[4] Fudan Univ, State Key Lab ASIC & Syst, Shanghai 200433, Peoples R China
[5] Shanxi Univ, Collaborat Innovat Ctr Extreme Opti, Taiyuan 030006, Shanxi, Peoples R China
[6] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Transducer Technol, Shanghai 200050, Peoples R China
关键词
VANADIUM DISULFIDE NANOSHEETS; CHEMICAL-VAPOR-DEPOSITION; REDUCED GRAPHENE OXIDE; HIGH-PERFORMANCE; MICRO-SUPERCAPACITORS; NANOSTRUCTURES; ELECTRODES; DISELENIDE; DICHALCOGENIDES;
D O I
10.1039/c8ta00089a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Metallic two-dimensional (2D) 1T-VSe2 with high conductivity and a large specific surface area is a promising electrode material for supercapacitors. Here, we use a facile chemical vapor deposition (CVD) method to prepare thin VSe2 nanosheets. A flexible in-plane solid-state supercapacitor is fabricated using the high-quality VSe2 nanosheets as the electrode material. The prepared supercapacitor presents an electrical double-layer capacitive behavior, and it has a high power density that is comparable with that of advanced graphene-based supercapacitors. The flexible supercapacitor also shows good mechanical stability to both bending and fatigue tests up to 10 000 cycles. This work provides a novel method for the fabrication of high-performance thin-film power sources, and paves the way for their application in soft thin-geometry devices.
引用
收藏
页码:8299 / 8306
页数:8
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