Synergistically Directed Assembly of Aromatic Stacks Based Metal-Organic Frameworks by Donor-Acceptor and Coordination Interactions

被引：34
作者：
Wang, Xi [1 ]
Zhang, Ying [4 ]
Chang, Ze [1 ,3 ]
Huang, Hui [1 ,3 ]
Liu, Xiao-Ting [1 ,3 ]
Xu, Jialiang [1 ]
Bu, Xian-He [1 ,2 ,3 ]
机构：
[1] Nankai Univ, Sch Mat Sci & Engn, Natl Inst Adv Mat, Tianjin Key Lab Met & Mol Based Mat Chem, Tianjin 300350, Peoples R China
[2] Nankai Univ, State Key Lab Elementoorgan Chem, Coll Chem, Tianjin 300071, Peoples R China
[3] Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China
[4] Hebei Univ Technol, Sch Chem Engn & Technol, Tianjin 300130, Peoples R China
来源：
CHINESE JOURNAL OF CHEMISTRY | 2019年 / 37卷 / 09期
基金：
中国博士后科学基金; 中国国家自然科学基金;
关键词：
LIGHT-HYDROCARBONS; ADSORPTION; SEPARATION; STABILITY; SORPTION; DESIGN; LUMINESCENT; MOLECULES; SURFACE;
D O I：
10.1002/cjoc.201900247
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A synergistically directed assembly approach to distinctive metal-organic frameworks utilizing both donor-acceptor (D-A) interaction from aromatic systems and coordination interactions is presented. Based on such an approach, the coronene-tpt (tpt = 2,4,6-tri(4-pyridyl)-1,3,5-triazine) stacks based coronene-MOF-1-4 have been successfully fabricated. Their structural discrepancies with coronene- absent control products, 1 '-4 ', illustrate clearly the significance of coronene-tpt based D-A interactions in these architectures. All these coronene-MOFs contain varied coronene-tpt stacks as organic secondary building blocks (SBUs), which are closely interrelated with the coordination based framework structures. Moreover, porous coronene-MOF-1 and -2 exhibit high physicochemical stability and significant light hydrocarbons storage and separation performances.
引用
收藏
页码：871 / 877
页数：7
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