Nonlinear optical waveguides in As2S3-Ag2S chalcogenide glass thin films

被引:21
作者
Almeida, J. M. P. [1 ,2 ]
Barbano, E. C. [1 ]
Arnold, C. B. [2 ]
Misoguti, L. [1 ]
Mendonca, C. R. [1 ]
机构
[1] Univ Sao Paulo, Sao Carlos Inst Phys, POB 369, BR-13560970 Sao Carlos, SP, Brazil
[2] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA
基金
巴西圣保罗研究基金会;
关键词
AG2S QUANTUM-DOT; FEMTOSECOND; PHOTONICS;
D O I
10.1364/OME.7.000093
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Chalcogenide glasses (ChGs) are promising materials for nonlinear optical applications due to their elevated third-order optical susceptibility. Nonetheless, oxidation and photorefractive effects make the characterization and processing of this class of materials an intricate process. Employing ultrashort laser pulses, we were able to investigate the optical nonlinearities of As2S3 thin films doped with Ag2S nanocrystals, as well as produce channel waveguides. The results showed that the nonlinear refractive indexes of these films are in the order of 2.3-5.2 x 10(-18) m(2)/W at wavelengths in the range of 775-1600 nm. Such film revealed to be proper for the development of nonlinear optical devices, since we have demonstrated the functionality of an 8.7 mm long waveguide for spectral broadening femtosecond IR pulses. (C) 2016 Optical Society of America
引用
收藏
页码:93 / 99
页数:7
相关论文
共 23 条
[1]   Metallic nanoparticles grown in the core of femtosecond laser micromachined waveguides [J].
Almeida, J. M. P. ;
Ferreira, P. H. D. ;
Manzani, D. ;
Napoli, M. ;
Ribeiro, S. J. L. ;
Mendonca, C. R. .
JOURNAL OF APPLIED PHYSICS, 2014, 115 (19)
[2]   Single-step synthesis of silver sulfide nanocrystals in arsenic trisulfide [J].
Almeida, Juliana M. P. ;
Lu, Chao ;
Mendonca, Cleber R. ;
Arnold, Craig B. .
OPTICAL MATERIALS EXPRESS, 2015, 5 (08) :1815-1821
[3]   Comparison of nonlinear-optical properties of sulfide glasses in bulk and thin film form [J].
Cerqua-Richardson, KA ;
McKinley, JM ;
Lawrence, B ;
Joshi, S ;
Villeneuve, A .
OPTICAL MATERIALS, 1998, 10 (02) :155-159
[4]  
Chichkov BN, 1996, APPL PHYS A-MATER, V63, P109, DOI 10.1007/BF01567637
[5]   Chalcogenide photonics [J].
Eggleton, Benjamin J. ;
Luther-Davies, Barry ;
Richardson, Kathleen .
NATURE PHOTONICS, 2011, 5 (03) :141-148
[6]   An alternative procedure for the determination of the optical band gap and thickness of amorphous carbon nitride thin films [J].
Escobar-Alarcon, L. ;
Arrieta, A. ;
Camps, E. ;
Muhl, S. ;
Rodil, S. ;
Vigueras-Santiago, E. .
APPLIED SURFACE SCIENCE, 2007, 254 (01) :412-415
[7]   Supercontinuum generation in the mid-infrared from a dispersion-engineered As2S3 glass rib waveguide [J].
Gai, Xin ;
Choi, Duk-Yong ;
Madden, Steve ;
Yang, Zhiyong ;
Wang, Rongping ;
Luther-Davies, Barry .
OPTICS LETTERS, 2012, 37 (18) :3870-3872
[8]   Femtosecond laser micromachining in transparent materials [J].
Gattass, Rafael R. ;
Mazur, Eric .
NATURE PHOTONICS, 2008, 2 (04) :219-225
[9]   Nonlinear optical properties of silver-doped As2S3 [J].
Kosa, T.I. ;
Rangel-Rojo, R. ;
Hajto, E. ;
Ewen, P.J.S. ;
Owen, A.E. ;
Kar, A.K. ;
Wherrett, B.S. .
Journal of Non-Crystalline Solids, 1993, 164-66 (pt 2) :1219-1222
[10]   Optical and catalytic properties of Ag2S nanoparticles [J].
Kryukov, AI ;
Stroyuk, AL ;
Zin'chuk, NN ;
Korzhak, AV ;
Kuchmii, SY .
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2004, 221 (1-2) :209-221