High-contrast sub-millivolt inelastic X-ray scattering for nano- and mesoscale science

被引:38
作者
Shvyd'ko, Yuri [1 ]
Stoupin, Stanislav [1 ]
Shu, Deming [1 ]
Collins, Stephen P. [2 ]
Mundboth, Kiran [2 ]
Sutter, John [2 ]
Tolkiehn, Martin [3 ]
机构
[1] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[2] Diamond Light Source Ltd, Didcot OX11 0DE, Oxon, England
[3] DESY, D-22607 Hamburg, Germany
关键词
GLASS-FORMING LIQUIDS; MEV ENERGY RESOLUTION; MICROSCOPIC DYNAMICS; SPECTROSCOPY; FRAGILITY; ALUMINUM; MODES; WATER;
D O I
10.1038/ncomms5219
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Photon and neutron inelastic scattering spectrometers are microscopes for imaging condensed matter dynamics on very small length and time scales. Inelastic X-ray scattering permitted the first quantitative studies of picosecond nanoscale dynamics in disordered systems almost 20 years ago. However, the nature of the liquid-glass transition still remains one of the great unsolved problems in condensed matter physics. It calls for studies at hitherto inaccessible time and length scales, and therefore for substantial improvements in the spectral and momentum resolution of the inelastic X-ray scattering spectrometers along with a major enhancement in spectral contrast. Here we report a conceptually new spectrometer featuring a spectral resolution function with steep, almost Gaussian tails, sub-meV (similar or equal to 620 mu eV) bandwidth and improved momentum resolution. The spectrometer opens up uncharted space on the dynamics landscape. New results are presented on the dynamics of liquid glycerol, in the regime that has become accessible with the novel spectrometer.
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页数:6
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