Preparing attosecond coherences by strong-field ionization

被引:31
作者
Pabst, Stefan [1 ,2 ]
Lein, Manfred [3 ,4 ]
Woerner, Hans Jakob [5 ]
机构
[1] DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany
[2] Harvard Smithsonian Ctr Astrophys, Inst Theoret Atom & Mol Phys, Cambridge, MA 02138 USA
[3] Leibniz Univ Hannover, Inst Theoret Phys, D-30167 Hannover, Germany
[4] Leibniz Univ Hannover, Ctr Quantum Engn & Space Time Res QUEST, D-30167 Hannover, Germany
[5] ETH, Lab Phys Chem, CH-8093 Zurich, Switzerland
基金
欧洲研究理事会;
关键词
MULTIPHOTON IONIZATION; CHARGE MIGRATION; LASER CONTROL; DYNAMICS; ATOMS; IONS;
D O I
10.1103/PhysRevA.93.023412
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Strong-field ionization (SFI) has been shown to prepare wave packets with few-femtosecond periods. Here, we explore whether this technique can be extended to the attosecond time scale. We introduce an intuitive model, which is based on the Fourier transform of the subcycle SFI rate, for predicting the bandwidth of ionic states that can be coherently prepared by SFI. The coherent bandwidth decreases considerably with increasing central wavelength of the ionizing pulse but it is much less sensitive to its intensity. Many-body calculations based on time-dependent configuration-interaction singles support these results. The influence of channel interactions and laser-induced dynamics within the ion is discussed. Our results further predict that multicycle femtosecond pulses can coherently prepare subfemtosecond wave packets with higher selectivity and versatility compared to single-cycle pulses with an additional sensitivity to the mutual parity of the prepared states.
引用
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页数:5
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