Design of a POSS-modified Zeolite Structure and the Study of the Enhancement of Ammonia-nitrogen Removal from Drinking Water

被引:1
|
作者
Lin, Derong [1 ,2 ]
Hu, Lijiang [2 ]
Zhang, Qun [2 ]
You, Hong [1 ]
机构
[1] Harbin Inst Technol, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China
[2] Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China
来源
MOLECULAR ENVIRONMENTAL SOIL SCIENCE AT THE INTERFACES IN THE EARTH'S CRITICAL ZONE | 2010年
关键词
WASTE-WATER; EXCHANGE;
D O I
10.1007/978-3-642-05297-2_36
中图分类号
S15 [土壤学];
学科分类号
0903 ; 090301 ;
摘要
In this work, the mesoporous zeolite molecular sieve (ZMS) surface was modified using polyhedral Coors) silsesquioxane (POSS) with carboxyl sodium terminal groups (POSS-COONa) as ion-exchange active groups. The characterization of the POSS-COONa structure by standard techniques (such as SEM, TEM, XRD, etc.) was investigated and discussed. With this approach, the exchange capacity of ammonia -nitrogen (NH3-N) in water would be greatly increased. The diffusion behavior of NH3-N in the pores of PUSS-modified ZMS was calculated using a molecular dynamic simulation (MDS) program of the Materials Stutio (MS) software which facilitate to study the effect of PUSS modification on pore structure and exchange capacity. The interface binding energy between POSS-ama and ZMS was calculated using MDS, facilitating the study of a simple regeneration method for exchanged active groups. It was estimated that the weight of the POSS-modified ZMS could be reduced by 25% for the same 90% of NH3-N removal rate of the normal ZMS under the same conditions. If the removal rate of the normal ZMS for a higher concentration of NH3-N in water was 60%similar to 70%, the removal rate of the POSSmodified ZMS could be up to 80%similar to 90%.
引用
收藏
页码:118 / 120
页数:3
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