A method of improving classification precision based on model population analysis of steel material for laser-induced breakdown spectroscopy

被引:9
作者
Xu, Lin [1 ]
Liang, Long [1 ]
Zhang, Tianlong [1 ]
Tang, Hongsheng [1 ]
Wang, Kang [2 ]
Li, Hua [1 ]
机构
[1] NW Univ Xian, Coll Chem & Mat Sci, Inst Analyt Sci, Xian 710069, Peoples R China
[2] Changan Univ, Coll Sci, Xian 710064, Peoples R China
基金
中国国家自然科学基金;
关键词
SUPPORT VECTOR MACHINE; NEURAL-NETWORKS; LIBS; IDENTIFICATION; SPECTROMETRY; FEASIBILITY; DIAGNOSTICS; POLYMERS; INDUSTRY; SURFACE;
D O I
10.1039/c4ay01557f
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
A novel method of improving classification precision, i.e. accuracy influence analysis (AIA), combined with support vector machines (SVM) is proposed for selecting informative variables of laser-induced breakdown spectroscopy (LIBS) spectra. Based on model population analysis (MPA), AIA could reveal informative variables that have statistically significant influence on the prediction accuracy of SVM sub-models. Support vector machine is then employed to build a more robust model and classify nine types of round steel based on the selected spectral variables. In this way, the classification performance of SVM is further improved and the computation time is reduced greatly. AIA is demonstrated to be a good alternative for the variable selection of high-dimensional LIBS dataset.
引用
收藏
页码:8374 / 8379
页数:6
相关论文
共 44 条
  • [1] [Anonymous], 2004, KERNEL METHODS PATTE
  • [2] [Anonymous], 2006, Handbook of Laser-Induced Breakdown Spectroscopy
  • [3] Beatrice S., 2005, SPECTROCHIM ACTA B, V60, P805
  • [4] Pigment analysis in Bronze Age Aegean and Eastern Mediterranean painted plaster by laser-induced breakdown spectroscopy (LIBS)
    Brysbaert, Ann
    Melessanaki, Krystalia
    Anglos, Demetrios
    [J]. JOURNAL OF ARCHAEOLOGICAL SCIENCE, 2006, 33 (08) : 1095 - 1104
  • [5] Diagnostics of high-temperature steel pipes in industrial environment by laser-induced breakdown spectroscopy technique: the LIBSGRAIN project
    Bulajic, D
    Cristoforetti, G
    Corsi, M
    Hidalgo, M
    Legnaioli, S
    Palleschi, V
    Salvetti, A
    Tognoni, E
    Green, S
    Bates, D
    Steiger, A
    Fonseca, J
    Martins, J
    McKay, J
    Tozer, B
    Wells, D
    Wells, R
    Harith, MA
    [J]. SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2002, 57 (07) : 1181 - 1192
  • [6] Christianini N., 2000, INTRO SUPPORT VECTOR, P189
  • [7] Laser-induced breakdown spectroscopy analysis of energetic materials
    De Lucia, FC
    Harmon, RS
    McNesby, KL
    Winkel, RJ
    Miziolek, AW
    [J]. APPLIED OPTICS, 2003, 42 (30) : 6148 - 6152
  • [8] Feasibility of detection and identification of individual bioaerosols using laser-induced breakdown spectroscopy
    Dixon, PB
    Hahn, DW
    [J]. ANALYTICAL CHEMISTRY, 2005, 77 (02) : 631 - 638
  • [9] Methodologies for laboratory Laser Induced Breakdown Spectroscopy semi-quantitative and quantitative analysis-A review
    Fantoni, R.
    Caneve, L.
    Colao, F.
    Fornarini, L.
    Lazic, V.
    Spizzichino, V.
    [J]. SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2008, 63 (10) : 1097 - 1108
  • [10] Laser-Induced Breakdown Spectroscopy
    Fortes, Francisco J.
    Moros, Javier
    Lucena, Patricia
    Cabalin, Luisa M.
    Javier Laserna, J.
    [J]. ANALYTICAL CHEMISTRY, 2013, 85 (02) : 640 - 669