Effectiveness of short-term air quality emission controls: a high-resolution model study of Beijing during the Asia-Pacific Economic Cooperation (APEC) summit period

被引:29
|
作者
Ansari, Tabish Umar [1 ]
Wild, Oliver [1 ]
Li, Jie [2 ]
Yang, Ting [2 ]
Xu, Weiqi [2 ,3 ]
Sun, Yele [2 ,3 ,4 ]
Wang, Zifa [2 ]
机构
[1] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England
[2] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China
[3] Univ Chinese Acad Sci, Coll Earth Sci, Beijing, Peoples R China
[4] Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen, Fujian, Peoples R China
基金
中国国家自然科学基金; 英国自然环境研究理事会;
关键词
FINE PARTICULATE MATTER; TIANJIN-HEBEI; SEVERE HAZE; BOUNDARY-LAYER; NORTH CHINA; PM2.5; CONCENTRATIONS; SOURCE APPORTIONMENT; POLLUTION EPISODES; RADIATIVE-TRANSFER; AEROSOL;
D O I
10.5194/acp-19-8651-2019
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We explore the impacts of short-term emission controls on haze events in Beijing in OctoberNovember 2014 using high-resolutionWeather Research and Forecasting model with Chemistry (WRF-Chem) simulations. The model reproduces surface temperature and relative humidity profiles over the period well and captures the observed variations in key atmospheric pollutants. We highlight the sensitivity of simulated pollutant levels to meteorological variables and model resolution and in particular to treatment of turbulent mixing in the planetary boundary layer. We note that simulating particle composition in the region remains a challenge, and we overpredict NH4 and NO3 at the expense of SO4. We find that the emission controls implemented for the Asia-Pacific Economic Cooperation (APEC) summit period made a relatively small contribution to improved air quality (20 %-26 %), highlighting the important role played by favourable meteorological conditions over this period. We demonstrate that the same controls applied under less favourable meteorological conditions would have been insufficient in reducing pollutant levels to meet the required standards. Continued application of these controls over the 6-week period considered would only have reduced the number of haze days when daily mean fine particulate matter exceeds 75 mu g m(-3) from 15 to 13 d (days). Our study highlights the limitations of current emission controls and the need for more stringent measures over a wider region during meteo-rologically stagnant weather.
引用
收藏
页码:8651 / 8668
页数:18
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