Controllable growth of MoS2 nanosheets on TiO2 burst nanotubes and their photocatalytic activity

被引:13
作者
Jiang, Qiushi [1 ]
Wang, Shang [1 ]
Li, Xue [2 ]
Han, Zhaolian [1 ]
Zhao, Chunli [3 ]
Di, Tingting [4 ]
Liu, Siyuan [1 ]
Cheng, Zhiqiang [1 ]
机构
[1] Jilin Agr Univ, Coll Resources & Environm, Changchun 130118, Peoples R China
[2] Jilin Agr Univ, Coll Informat Technol, Changchun 130118, Peoples R China
[3] Jilin Agr Univ, Coll Hort, Changchun 130118, Peoples R China
[4] Northeast Elect Power Design Inst Co LTD, China Power Engn Consulting Grp, Changchun 130021, Peoples R China
关键词
CHARGE-CARRIER DYNAMICS; NANOROD HETEROSTRUCTURE; NOBLE-METAL; PERFORMANCE; ANATASE; NANOWIRES;
D O I
10.1039/d0ra08421b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
MoS2 nanosheets were grown on TiO2 nanotubes by the simple hydrothermal method for the first time. The layer-by-layer growth of MoS2 nanosheets led to a significant increase in the specific surface area of TiO2/MoS2 burst tube composites compared with TiO2 burst tubes, a significantly enhanced ability to separate photo-induced carriers, and synergistic adsorption and visible light catalytic activity of dye molecules. The maximum adsorption (q(max)) of MB was 72.46 mg g(-1). In addition, 94.1% of MB could be degraded after 30 minutes of visible light irradiation. The microsurface morphology, structure, chemical composition, element valence and band width of TiO2/MoS2 nanocomposites were analyzed by scanning electron microscopy (SEM), transmission electron microscopy (TEM), energy dispersive X-ray spectroscopy (EDS), X-ray photoelectron spectroscopy (XRD), X-ray photoelectron spectroscopy (XPS), diffuse reflectance spectroscopy (DRS) and photoluminescence spectroscopy (PL). The mechanism of photocatalytic reaction was studied via free radical capture experiments.
引用
收藏
页码:40904 / 40915
页数:12
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