Probing atomic positions of adsorbed ammonia molecules in zeolite

被引:27
作者
Ye, Lin [1 ]
Lo, Benedict T. W. [1 ]
Qu, Jin [1 ]
Wilkinson, Ian [2 ]
Hughes, Tim [2 ]
Murray, Claire A. [3 ]
Tang, Chiu C. [3 ]
Tsang, Shik Chi Edman [1 ]
机构
[1] Univ Oxford, Dept Chem, Wolfson Catalysis Ctr, S Parks Rd, Oxford OX1 3QR, England
[2] Siemens Plc, CT NTF, Wharf Rd, Oxford OX29 4BP, England
[3] Diamond Light Source Ltd, Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England
基金
英国工程与自然科学研究理事会;
关键词
SELECTIVE CATALYTIC-REDUCTION; LEWIS-ACID SITES; FE-ZSM-5; CATALYSTS; SOLID-STATE; H-ZSM-5; ZSM-5; NO; PERFORMANCE; ADSORPTION; FRAMEWORK;
D O I
10.1039/c5cc10476a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Atomic positions and interactions between adsorbed guest molecules, such as ammonia in H-ZSM-5 microporous solids, are for the first time revealed by making use of the change in the periodical scattering parameter using in situ synchrotron powder X-ray diffraction combined with refinement within experimental errors.
引用
收藏
页码:3422 / 3425
页数:4
相关论文
共 23 条
[1]   Methanol to gasoline over zeolite H-ZSM-5: Improved catalyst performance by treatment with NaOH [J].
Bjorgen, Morten ;
Joensen, Finn ;
Holm, Martin Spangsberg ;
Olsbye, Unni ;
Lillerud, Karl-Petter ;
Svelle, Stian .
APPLIED CATALYSIS A-GENERAL, 2008, 345 (01) :43-50
[2]   Conversion of methanol to hydrocarbons over zeolite H-ZSM-5: On the origin of the olefinic species [J].
Bjorgen, Morten ;
Svelle, Stian ;
Joensen, Finn ;
Nerlov, Jesper ;
Kolboe, Stein ;
Bonino, Francesca ;
Palumbo, Luisa ;
Bordiga, Silvia ;
Olsbye, Unni .
JOURNAL OF CATALYSIS, 2007, 249 (02) :195-207
[3]   Metal-organic frameworks with high capacity and selectivity for harmful gases [J].
Britt, David ;
Tranchemontagne, David ;
Yaghi, Omar M. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2008, 105 (33) :11623-11627
[4]   Acidic Strengths of Bronsted and Lewis Acid Sites in Solid Acids Scaled by 31P NMR Chemical Shifts of Adsorbed Trimethylphosphine [J].
Chu, Yueying ;
Yu, Zhiwu ;
Zheng, Anmin ;
Fang, Hanjun ;
Zhang, Hailu ;
Huang, Shing-Jong ;
Liu, Shang-Bin ;
Deng, Feng .
JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (15) :7660-7667
[5]  
Doonan CJ, 2010, NAT CHEM, V2, P235, DOI [10.1038/nchem.548, 10.1038/NCHEM.548]
[6]   How a century of ammonia synthesis changed the world [J].
Erisman, Jan Willem ;
Sutton, Mark A. ;
Galloway, James ;
Klimont, Zbigniew ;
Winiwarter, Wilfried .
NATURE GEOSCIENCE, 2008, 1 (10) :636-639
[7]   SOLID-STATE NUCLEAR-MAGNETIC-RESONANCE STUDIES OF ACID SITES IN ZEOLITES [J].
FREUDE, D ;
ERNST, H ;
WOLF, I .
SOLID STATE NUCLEAR MAGNETIC RESONANCE, 1994, 3 (05) :271-286
[8]   Adsorption equilibria of ammonia gas on inorganic and organic sorbents at 298.15 K [J].
Helminen, J ;
Helenius, J ;
Paatero, E ;
Turunen, I .
JOURNAL OF CHEMICAL AND ENGINEERING DATA, 2001, 46 (02) :391-399
[9]   STRUCTURE OF SYNTHETIC ZEOLITE ZSM-5 [J].
KOKOTAILO, GT ;
LAWTON, SL ;
OLSON, DH ;
OLSON, DH ;
MEIER, WM .
NATURE, 1978, 272 (5652) :437-438
[10]   ELECTRONIC-STRUCTURE CALCULATIONS OF AMMONIA ADSORPTION IN H-ZSM-5 ZEOLITES [J].
KYRLIDIS, A ;
COOK, SJ ;
CHAKRABORTY, AK ;
BELL, AT ;
THEODOROU, DN .
JOURNAL OF PHYSICAL CHEMISTRY, 1995, 99 (05) :1505-1515