Profiles and Risk Assessment of Organochlorine Pesticides in Three Gorges Reservoir, China

被引：10
作者：
Yang, Yuyi [1 ]
Liu, Minxia [1 ,2 ]
Yun, Xiaoyan [1 ,2 ]
Ge, Jing [1 ]
Wang, Jun [1 ]
机构：
[1] Chinese Acad Sci, Key Lab Aquat Bot & Watershed Ecol, Wuhan Bot Garden, Wuhan 430074, Peoples R China
[2] Univ Chinese Acad Sci, Beijing, Peoples R China
来源：
CLEAN-SOIL AIR WATER | 2017年 / 45卷 / 02期
关键词：
Aquatic pollution; DDTs; HCHs; Heptachlor; Risk assessment; POLYCYCLIC AROMATIC-HYDROCARBONS; YANGTZE-RIVER; SURFACE WATERS; HUAIHE RIVER; EAST CHINA; SEDIMENTS; RESIDUES; SOIL; DDT; CONTAMINANTS;
D O I：
10.1002/clen.201600823
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
The environmental pollution of the Three Gorges Reservoir in China may not be desirable and has adverse effects on biodiversity and human health in this region. Concentrations of 16 organochlorine pesticides (OCPs) were investigated in 19 surface water samples collected from near dam region of the Three Gorges Reservoir. The concentrations of total OCPs ranged from 14 to 88 ng L-1 with a geometric mean of 23 ng L-1. The spatial distribution of OCPs concentrations indicated the giant reservoir was sink of OCPs for upstream as well as source for downstream. The mean concentrations of total hexachlorocyclohexanes (HCHs) and dichlorodiphenyltrichloroethanes (DDTs) were 10 and 9.7 ng L (1), respectively. Historical use of lindane and DDT was found to be the primary source of HCHs and DDTs. The ratio between heptachlor and its metabolic products indicated new input of heptachlor occurred in this region. Among the 16 detected OCPs, the cancer risks for human of heptachlor and heptachlorepoxide were all above 10(-4), indicating a potential threat of the two OCPs to human health.
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页数：7
相关论文
共 40 条
[31]   Endosulfan, a global pesticide: A review of its fate in the environment and occurrence in the Arctic [J].
Weber, Jan ;
Halsall, Crispin J. ;
Muir, Derek ;
Teixeira, Camilla ;
Small, Jeff ;
Solomon, Keith ;
Hermanson, Mark ;
Hung, Hayley ;
Bidleman, Terry .
SCIENCE OF THE TOTAL ENVIRONMENT, 2010, 408 (15) :2966-2984
[32]  
WHO, 1979, DDT ITS DER
[33]   Differential toxicity and environmental fates of hexachlorocyclohexane isomers [J].
Willett, KL ;
Ulrich, EM ;
Hites, RA .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (15) :2197-2207
[34]  
Wu L, 2011, 3 INT C ENV SCI IN B, V10, P1496, DOI DOI 10.1016/J.PR0ENV.2011.09.238
[35]   Residues of organochlorine pesticides in near shore waters of LaiZhou Bay and JiaoZhou Bay, Shandong Peninsula, China [J].
Xu, Xiaoqin ;
Yang, Huanghao ;
Li, Qinghng ;
Yang, Baijuan ;
Wang, Xiaoru ;
Lee, Frank S. C. .
CHEMOSPHERE, 2007, 68 (01) :126-139
[36]   Occurrence and distribution of organochlorine pesticides (HCH and DDT) in sediments collected from East China Sea [J].
Yang, RQ ;
Jiang, GB ;
Zhou, QF ;
Yuan, CG ;
Shi, JB .
ENVIRONMENT INTERNATIONAL, 2005, 31 (06) :799-804
[37]   Soil nitrogen dynamics following short-term revegetation in the water level fluctuation zone of the Three Gorges Reservoir, China [J].
Ye, Chen ;
Cheng, Xiaoli ;
Zhang, Yulong ;
Wang, Zhixi ;
Zhang, Quanfa .
ECOLOGICAL ENGINEERING, 2012, 38 (01) :37-44
[38]   Occurrence of PAHs, PCBs and organochlorine pesticides in the Tonghui River of Beijing, China [J].
Zhang, ZL ;
Huang, J ;
Yu, G ;
Hong, HS .
ENVIRONMENTAL POLLUTION, 2004, 130 (02) :249-261
[39]   Polychlorinated biphenyl congeners and organochlorine insecticides in the water column and sediments of Daya Bay, China [J].
Zhou, JL ;
Maskaoui, K ;
Qiu, YW ;
Hong, HS ;
Wang, ZD .
ENVIRONMENTAL POLLUTION, 2001, 113 (03) :373-384
[40]   Levels and source of organochlorine pesticides in surface waters of Qiantang River, China [J].
Zhou, Rongbing ;
Zhu, Lizhong ;
Chen, Yuyun .
ENVIRONMENTAL MONITORING AND ASSESSMENT, 2008, 136 (1-3) :277-287
1234