Recent achievements on middle and far-infrared second-order nonlinear optical materials

被引：383
作者：
Guo, Sheng-Ping [1 ]
Chi, Yang [1 ]
Guo, Guo-Cong [2 ]
机构：
[1] Yangzhou Univ, Coll Chem & Chem Engn, Yangzhou 225002, Jiangsu, Peoples R China
[2] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
来源：
COORDINATION CHEMISTRY REVIEWS | 2017年 / 335卷
关键词：
Chalcogenides; Halides; Iodates; Crystal structure; NLO property; Functional moiety theory; STRONG 2ND-HARMONIC GENERATION; LASER DAMAGE THRESHOLD; DIAMOND-LIKE SEMICONDUCTORS; PHASE-CHANGE PROPERTIES; DIRECT-BAND-GAP; IR REGION; CRYSTAL-STRUCTURE; NONCENTROSYMMETRIC COMPOUNDS; QUATERNARY CHALCOGENIDES; SHG MATERIALS;
D O I：
10.1016/j.ccr.2016.12.013
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
The exploration and development of second-order nonlinear optical (NLO) materials in the middle- and far infrared (MFIR) region are important and high profile topics in the fields of NLO, solid-state chemistry and laser. Common MFIR NLO materials are chalcogenides, halides, and iodates, which have a wide MFIR transparent range and large NLO coefficients. This review summarizes recent achievements on MFIR NLO materials, and specifically focuses on their crystal structures and NLO properties. Compared to known materials, the common choice for cations are alkali-metal Li, Na, K, Rb and Cs, the coin-metal Ag, and the alkali-earth metal Ba. Exploring mixed-anions materials could be one of the most promising solutions to obtaining NLO materials with both large second-harmonic generation (SHG) intensities and high laser induced damage thresholds (LIDTs). This review also summarizes functional moiety theory to elucidate the design of promising NLO materials. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码：44 / 57
页数：14
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